Metallogenetic regularity and prospecting direction of granite related Li-Be-Nb-Ta deposits in the Nanling region, South China
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摘要:
南岭是全球最重要的稀有和有色金属资源基地之一, 以大面积出露的花岗质岩浆岩与大规模的稀有金属矿化而举世瞩目。华南多旋回构造岩浆活动, 造就了广泛发育的各类花岗岩, 并普遍经历了高分异作用, 使得钨、锡、锂、铍、铌、钽等稀有金属不同程度富集成矿。前人对南岭钨和锡的时空分布规律、成矿作用和成矿动力学背景进行了大量研究。本文结合近年矿产调查新进展, 重点总结了南岭花岗岩区锂铍铌钽矿化类型、时空分布规律及其成矿条件, 系统梳理了锂铍铌钽矿化相关花岗岩的成矿专属性。花岗质岩浆体系中源区组成、部分熔融程度、结晶分异程度、岩浆-热液流体的交代作用控制着锂、铍、铌、钽的分配和富集, 铌和钽可在花岗质岩浆熔体演化晚期阶段形成独立矿物, 铍一般在岩浆-热液的过渡阶段富集, 锂在伟晶岩阶段形成锂辉石, 也可富集于流体中交代形成锂云母。南岭地区铌钽矿化主要产出在花岗岩晚期阶段和云英岩中, 铍常与钨锡相伴生产出于石英脉型和接触交代型矿床中, 南岭锂资源以锂云母形式主要产出于富锂花岗岩体的云英岩化带。本文进一步讨论了多期岩浆作用与铌钽成矿关系、岩浆热液体系中铍与钨锡的成矿机理及南岭花岗岩区锂(锂云母)的成矿潜力, 这对下一步南岭地区锂铍铌钽找矿行动部署具有重要的意义。
Abstract:The Nanling region is one of the world's most essential rare and non-ferrous mineral resource bases, characterized by abundant highly fractionated granitic rocks exposed accompanied with significant rare metal mineralization, including W, Sn, Li, Be, Nb, Ta, which were due to the multiple tectono-magmatic events. The spatial-temporal distribution, mineralization and metallogenic dynamics of W and Sn in the Nanling region have been studied by previous studies. Based on the latest exploration progress in the Nanling region, this paper reviews the mineralization type, temporal and spatial distribution of Li-Be-Nb-Ta deposits and their relationship with highly fractionated granites, and summarize the metallogenic specialization of granites related to Li-Be-Nb-Ta mineralization. The distribution and enrichment of Li, Be, Nb, Ta is controlled by composition of source, partial melting crystallization differentiation and the alternation of magma-hydrothermal fluid in granitic magma system. Nb and Ta generally aggregate in the late stage of magmatic evolution. Be tends to be enriched in the magma-hydrothermal transition stage. Li forms spodumene at the pegmatite stage, and can also be enriched in the hydrothermal fluid metasomatism to form lepidolite. In the Nanling region, Nb-Ta mineralization is mainly hosted in greisens and top of granites. Be and W-Sn mineralization are hosted in quartz-vein type deposits and contact metasomatic type deposits. Li resources are mainly hosted in greisenization zone of Li-rich granites. This paper further discusses the relationship between multi-stage magmatic activities and Nb-Ta mineralization, the mineralization mechanism of Be and W-Sn in magmatic-hydrothermal system, and the potential of Li mineralization in Nanling region, which is of great significance for the Li-Be-Nb-Ta prospecting in this region.
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图 1
南岭及邻区花岗岩和Li-Be-Nb-Ta矿床空间分布图(据孙涛, 2006; 赵正等, 2022)
Figure 1.
The distribution map of granite and Li-Be-Nb-Ta deposits in the Nanling and its adjacent region, South China (after Sun, 2006; Zhao et al., 2022)
图 2
南岭及邻区Li-Be-Nb-Ta矿床的时代分布图
Figure 2.
Age distribution of the Li-Be-Nb-Ta deposits in the Nanling and its adjacent region, South China
图 4
大吉山W-Be-Nb-Ta矿床成矿模式图(据Wu et al., 2017)
Figure 4.
Metallogenic model of the Dajishan W-Be-Nb-Ta deposit (after Wu et al., 2017)
图 6
柿竹园W-Sn-Mo-Bi-Be矿床矿化模式图(据Zhao et al., 2021a)
Figure 6.
Metallogenic model of Shizhuyuan W-Sn-Mo-Bi-Be deposit (after Zhao et al., 2021a)
图 7
南平伟晶岩矿床剖面图(a)和31号花岗伟晶岩脉内部结构图(b)(据Tang et al., 2017)
Figure 7.
The cross-section map (a) and No.31 granitic pegmatite vein internal textural zones (b) of the Nanping pegmatite deposit (after Tang et al., 2017)
图 8
界牌岭Sn-F-Be-Nb-Ta-Li矿床成矿模式图(据许若潮等, 2022)
Figure 8.
Metallogenic model of the Jiepailing Sn-F-Be-Nb-Ta-Li deposit (after Xu et al., 2022)
图 9
南岭成锂铍铌钽矿花岗岩系列地球化学图解
Figure 9.
Geochemical diagrams of ore-forming granites related to Li, Be, Nb, Ta in the Nanling region
图 10
南岭与锂铍铌钽成矿相关花岗岩源区图解
Figure 10.
Plots of source region of Li-Be-Nb-Ta related granitoids in the Nanling region
图 11
南岭与锂铍铌钽成矿有关花岗岩类的分异演化图解
Figure 11.
Plots of differentiation and evolution of Li-Be-Nb-Ta related granitoids in the Nanling region
图 12
南岭与锂铍铌钽成矿相关花岗岩类球粒陨石标准化稀土元素配分图(标准化值据Sun and McDonough, 1989)
Figure 12.
Chondrite-normalized REE patterns of Li-Be-Nb-Ta related granitoids in the Nanling region (standardized value after Sun and McDonough, 1989)
图 13
南岭与锂铍铌钽成矿有关花岗岩类的Rb-(Y+Nb) (a)和Rb-(Yb+Ta) (b)图解(底图据Pearce et al., 1984)
Figure 13.
Plots of Rb vs. Y+Nb (a) and Rb vs. Yb+Ta (b) of Li-Be-Nb-Ta related granitoids in the Nanling region (after Pearce et al., 1984)
表 1
南岭稀有金属矿床主要类型、成矿时代、成矿元素和稀有金属矿物组合特征表
Table 1.
Major types, ore-forming ages, rare elements, and mineral assemblage of rare metal deposits in the Nanling region, South China
矿床类型 矿床名称 元素组合 大地构造位置 年龄(Ma) 矿物组合 岩浆属性 矿床规模 资料来源 花岗岩型 广西栗木 Sn-W-Nb-Ta-Li 桂北台隆越城岭断褶带 220 铌钽锰矿、钽铌锰矿、细晶石、锡石、黑钨矿 弱过铝-强过铝质 大型 杨锋等, 2009; 李胜虎等, 2015; Che et al., 2019 广西高岭 W-Nb-Ta-Li 桂北台隆越城岭断褶带 220、204 铌钽锰矿、钽铌锰矿、细晶石、黑钨矿 弱过铝-强过铝质 中型 张迪等, 2015; Che et al., 2019 江西大吉山 W-Sn-Nb-Ta-Be 赣湘桂粤褶皱带 161~151 铌锰矿、钽锡锰矿、铌钽锰矿、黑钨矿、白钨矿、绿柱石 弱过铝-强过铝质 中型 张思明等, 2011 湖南尖峰岭 Li-Nb-Ta 赣湘桂粤褶皱带 159 铌铁金红石、铌铁矿、钨铌铁矿、含铌黑钨矿、黑稀金矿、富铌锡石、黑钨矿 强过铝质 大型 文春华等, 2017 湖南金竹垄 W-Be-Ta-Nb-Li 赣湘桂粤褶皱带 156~148 铌钽锰矿、细晶石、黑钨矿、日光榴石、绿柱石 弱过铝-强过铝质 大型 孙颖超等, 2017; Che et al., 2019 江西姜坑里 Li-Nb-Ta 南岭构造带与武夷断褶带的复合部位 141 铌铁矿、钽铁矿、钽锡矿、细晶石、(铁)锂云母 弱过铝-强过铝质 中型 司晓博等, 2020; 李晓峰等, 2021 江西旱叫山 Li-Nb-Ta 南岭构造带与武夷断褶带的复合部位 132 铌铁矿、钽铁矿、钽锡矿、细晶石、(铁)锂云母 弱过铝-强过铝质 中型 司晓博等, 2020; 李晓峰等, 2021 江西牛岭坳 Li-Nb-Ta 南岭构造带与武夷断褶带的复合部位 132 铌铁矿、钽铁矿、钽锡矿、细晶石、(铁)锂云母 弱过铝-强过铝质 大型 司晓博等, 2020; 李晓峰等, 2021 江西海螺岭 Li-Nb-Ta 南岭构造带与武夷断褶带的复合部位 128 铌铁矿、钽铁矿、钽锡矿、细晶石、(铁)锂云母 弱过铝-强过铝质 中型 司晓博等, 2020; 李晓峰等, 2021 湖南上堡 W-Nb-Ta 赣湘桂粤褶皱带 87 富铌金红石、铌铁矿、钨铌铁矿、黑钨矿 弱过铝-强过铝质 中型 Zhao et al., 2021b 云英岩-
花岗岩型广东良源 Nb-Ta-Rb-W 南岭东西向构造岩浆带与武夷山北东向构造带交汇部位 169~159 黑钨矿、白钨矿、锡石、富铌钽铷黑钨矿和锡石 弱过铝-强过铝质 大型 范飞鹏等, 2022 云英岩型 湖南正冲 Sn-W-Rb-Li-Cs-Nb-Ta 赣湘桂粤褶皱带 154~142 黑钨矿、锡石、铁锂云母、铌铁矿、铌钽锰矿 弱过铝-强过铝质 大型 文春华等, 2016 条纹岩型 湖南香花岭 Sn-Nb-Ta-Be-Li 赣湘桂粤褶皱带 158~151 金绿宝石、塔菲石、香花石、孟宪民石、硅铍石、锂铍石、锂霞石 弱过铝-强过铝质 中型 来守华, 2014; 赵一鸣等, 2017; Wu et al., 2022 矽卡岩型 湖南柿竹园 W-Sn-Mo-Bi-Be 赣湘桂粤褶皱带 153~151 白钨矿、辉钼矿、辉铋矿、黑钨矿、绿柱石、硅铍钇石、黑稀金矿 准铝-弱过铝质 大型 毛景文等, 2004; 王敏等, 2016 石英脉型 江西画眉坳 W-Be 南岭构造带与武夷断褶带的复合部位 157 黑钨矿、绿柱石 过铝质 中型 毛景文等, 2004; Feng et al., 2015 江西西华山 W-Sn-Be 赣湘桂粤褶皱带 155 黑钨矿、绿柱石 准铝-弱过铝质 中型 郭小飞等, 2022 江西漂塘 W-Mo-Be 赣湘桂粤褶皱带 152 黑钨矿、绿柱石 弱过铝质 小型 张文兰等, 2009 花岗伟晶岩型 江西西港 Li-Be-Nb-Ta 武夷山隆起区西段南缘 422 锂辉石、钽铌矿、铌钽铁矿、钽铌铁矿、绿柱石、锂云母、金红石、含钽锡石、褐钇铌矿等 弱过铝-强过铝质 大型 Che et al., 2019 福建西坑 Li-Be-Nb-Ta 闽西北加里东褶皱带东南段 391~387 铌铁矿、钽铁矿、锂辉石、磷锂铝石、磷铁锂矿、柱磷锶锂矿、绿柱石、红磷铍锰矿、磷铍钙石、硅铍石、羟硅铍石 弱过铝质 大型 Tang et al., 2017; Che et al., 2019 广东厚溪 Li-Nb-Ta 云开大山隆起区 248 铌钽铁矿、细晶石、钽锰矿、褐钇铌矿、磷铝锂石、绿柱石等 弱过铝-强过铝质 中型 Che et al., 2019 广东洞头南 Li-Nb-Ta 云开大山隆起区 246 铌钽铁矿、细晶石、钽锰矿、褐钇铌矿、磷铝锂石、绿柱石等 弱过铝-强过铝质 中型 Che et al., 2019 广东村心 Li-Nb-Ta 云开大山隆起区 246 铌钽铁矿、细晶石、钽锰矿、褐钇铌矿、磷铝锂石、绿柱石等 弱过铝-强过铝质 中型 Che et al., 2019 江西头陂 Li-Be-Nb-Ta 武夷山隆起区中段西缘 246 钽铌铁矿、铌钽铁矿、重钽铁矿、细晶石、锂辉石、锂云母、钛钽铌矿、绿柱石 弱过铝-强过铝质 中型 李晓峰等, 2021 广东深坑 Nb-Ta 云开大山隆起区 245 铌钽铁矿、细晶石、钽锰矿、褐钇铌矿、磷铝锂石、绿柱石等 弱过铝-强过铝质 中型 Che et al., 2019 江西河源 Li-Nb-Ta 武夷山隆起区中段西缘 220~200 钽铌铁矿、铌钽铁矿、重钽铁矿、细晶石、锂辉石、锂云母、钛钽铌矿、绿柱石 弱过铝-强过铝质 中型 胡为正等, 2005, 2006 花岗斑岩型 福建行洛坑 W-Be 闽西北加里东隆起带南段 151~143 白钨矿、黑钨矿、绿柱石 弱过铝-强过铝质 中型 张清清等, 2020; 申景辉, 2021 江西界牌岭 Sn-Be-Ta-Nb-Li 赣湘桂粤褶皱带 92~89 铌锰矿、铌钽矿、铌铁金红石、锡石、黑钨矿、铁锂云母、金绿宝石、日光榴石、羟硅铍石 弱过铝-强过铝质 大型 王艳丽等, 2014; Yuan et al., 2015; Che et al., 2019 
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