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Interplay between six wave mixing photonic band gap signal and second-order nonlinear signal in electromagnetically induced grating

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Abstract

For the first time, we experimentally and theoretically research about the second-order nonlinear signal (SNS) including electromagnetically induced absorbing (EIA) and electromagnetically induced gain (EIG), six wave mixing band gap signal (SWM BGS) resulting from photonic band gap structure in an inverted Y-type four level system with the electromagnetically induced grating. The interplay between the SNS and SWM BGS is illustrated clearly for the first time. When we change the frequency detuning to make the SWM BGS and SNS overlap, the SWM BGS is suppressed and the intensity of SNS is strongest near the resonance point. We can control the intensity of the SWM BGS and EIG caused by the classic effect through changing the power of coupling field. And the changes on the EIA generated by the quantum effect are obtained by changing the power of dressing field. Since the SWM BGS is the enhancement of the four wave mixing band gap signal (FWM BGS), when we set FWM BGS as the input and SNS as the modulation role to control the amplification amplitude for the FWM BGS in our scheme, the adjustable optical amplifier can be obtained.

© 2015 Optical Society of America

1. Introduction

Atomic coherence which can lead to a great many of significant physical phenomena is the result of interaction between light and materials. Recently, increasingly experimental researches are reported on the atomic coherence [1–3 ]. It is well-known that the six-wave mixing (SWM) is a nonlinear optical effect generated by lights with different frequencies and different quantum properties. In the nonlinear wave-mixing process, atomic coherence of the electromagnetically induced transparency (EIT) plays a critical role has been demonstrated experimentally and theoretically in recent researches [4–9 ]. Furthermore, the increasingly effect has been paid on the switch between EIT and electromagnetically induced absorption (EIA) [3,10 ]. In the EIT environment, SWM signal can transmit through the atomic medium and the fluorescence can be generated due to spontaneous emission [11–14 ]. And the EIT-based nonlinear schemes can be driven by traveling wave beams as well as by a standing wave (SW) which formed by the two same frequency counter propagating coupling fields [15,16 ]. Thus in an atomic system driven by two counter propagating coupling fields can obtain the large nonlinearity. It is reported that the electromagnetically induced grating [17,18 ] resulted from the interaction of the SW with the atomic coherent medium can possess photonic band gap (PBG) structure in a variety of interesting research results [19,20 ].

In this paper, the optical response of hot rubidium (85Rb) atoms driven by a SW is investigated in an inverted Y-type four level system and six wave mixing band gap signal (SWM BGS) and probe transmission signal are obtained firstly in the experiment. Especially, the two photon process including EIA and electromagnetically induced gain (EIG) are researched experimentally and theoretically for the first time. And we define the two photon process as the second-order nonlinear signals (SNS) in the paper. When we change the frequency detunings and the powers of the laser fields, the interplay between the SWM BGS and SNS as well as its application are also discussed for the first time in this paper. Furthermore, we also demonstrate the relation of the probe transmission signal and fluorescence in our research.

2. Experimental scheme

The experiment was completed in a rubidium atomic vapor cell of 85Rb. The energy levels 5S 1/2(F = 3) (|0>), 5S1/2(F = 2) (|3>), 5P3/2 (|1>) and 5D5/2 (|2>) compose a inverted-Y energy system as shown in Fig. 1(b) . Probe laser beam E1 (wavelength of 780.245 nm, frequency ω1 and wave vector k1) connects the transition 5S1/2 (F = 3) (|0>) to 5P3/2 (|1>). The laser beam E2 (wavelength of 775.978 nm, ω2, k2) drive an upper transition 5P3/2 (|1〉) to 5D5/2 (|2〉). A pair of coupling laser beams E3 (wavelength of 780.238 nm, ω3, k3) and 3 (wavelength of 780.238 nm, ω´3, k´3) connect the transition 5S1/2(F = 2) (|3〉) to 5P3/2 (|1〉. The coupling field E3 and 3 which propagate through 85Rb vapor in the opposite direction generate a standing wave Ec=y^[E3cos(ω3tk3x)+E3cos(ω3t+k3x)], which results into an EIG. Furthermore EIG will lead to a PBG structure as shown in Fig. 1(c). In addition, the intensity of probe beam E1 is the only weak laser beam while other laser beams are strong. As illustrated on Fig. 1(a), the weak probe beam E1 propagates through the 85Rb vapors in the same direction of 3 with a small angle between them. The dressing field E2 propagates in the opposite direction of E3 with a small angle between them. Due to the small angle between the probe beam E1 and the beam 3, the geometry not only satisfies the phase-matching (kS = k1 + k2−k2 + k3-k′3) also provides a convenient spatial separation of the applied laser and generated signal beams. Thus we can detect the generated beams with highly directional [21]. The generated SWM BGS satisfies the phase-matching kS = k1 + k2−k2 + k3-k′3. Besides SWM BGS, there also exists SNS in the reflection signal channel as shown in Fig. 1(a). The reflection signal and the probe transmission signal are detected by a photodiode and avalanche photodiode detectors respectively. In addition, three fluorescence signals caused by spontaneous decay are measured. The second order fluorescence R0 and fourth order fluorescence R1, R2 are generated due to the spontaneous emission from |1 and |2, respectively. Fluorescence signals are captured by another photodiode.

 figure: Fig. 1

Fig. 1 (a) The setup of our experiment. (b) Inverted-Y type energy system. (c) Schematic of an electromagnetically induced grating formed by two coupling beams E3 and E′3. (d) The single dressed energy level schematic diagrams and the calculated single dressed period energy levels. (e) The double dressed energy level schematic diagrams and the calculated double dressed periodic energy levels.

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It is the essential to the generation of the PBG structure that the medium should have a periodic refractive index. In order to get the periodic refractive index, the susceptibility of the medium should be periodic by considering the relation of the refractive index with the susceptibility, i.e.,n=1+Re(χ). Thus we must get the periodic energy level structure to generate the periodic susceptibility. Hence, the periodic energy levels can be obtained in Fig. 1(d)-1(e) by introducing periodic standing wave field. In Fig. 1(d), the level |1will be split into two dressed states|G30±. The two dressed states|G30± have the eigenvaluesλ|G30±=Δ/32±Δ32/4+|G30|2. And theλ|G30±|values are also periodic along x because |G30|2 is periodic along x-axis. Thus we can obtain the periodic energy levels as shown in Fig. 1(e). When E2 is turn on, due to the second level dressing effect of E2, |G30+is further split into two dressed states|G30+G2±. The two dressed states |G30+G2± have the eigenvaluesλ|G30+G±2=-Δ3+Δ32+4|G30|22+Δ2"±Δ2"2+4|G2|22with Δ2"2-{-Δ+3Δ32+4|G30|2}/2. Thus we also obtain the double dressed periodic energy levels as shown in Fig. 1(d)-1(e).

3. Results and discussions

First, we observe the probe transmission signal, reflection signal, and fluorescence when we block the different laser beam in case of scanning the frequency detuningΔ2in Fig. 2 . Figure 2(a) represents the changes on the probe transmission signal when different laser beams are blocked. When one block E3and E3 in Fig. 2(a1), there is a peak on the probe transmission signal locating at the position of Δ1=Δ2. And the peak stands for the enhancement of probe transmission signal caused by the term |G2|2/d20inρ10(1) (see Appendix). Next the beamE3is blocked in Fig. 2(a2), the peak is lower compared with the Fig. 2(a1) because of the strong cascade-dressing interaction between E3(E3) and E2 which leads to the suppression effect of E3 on the peak by considering the cascade-dressing term|G2|2/d20+|G30|2/d30inρ10(1). When we block the beamE1in Fig. 2(a3), the peak disappeared because the term G1=0 inρ10(1). When all laser beams are opened in Fig. 2(a4), we can find that the peak on the probe transmission signal becomes lower than peaks in Fig. 2(a1) and Fig. 2(a2). The reason is that the cascade interaction which results in the suppression effect of E3 on the peak plays a vital role on the intensity of peak. Figure 2(b) confirms the existence of SWM BGS and SNS in the reflection signal channel with the different laser beam blocked. Because the beamE2 propagates in the opposite direction of E1 in our experiment, the Doppler-free condition is satisfied in the subsystem |0|1|2 and the experimental setup will be in the EIT environment. So the EIT-induced EIG will be generated in the EIT environment. Figure 2(b) has two columns of signals and we observe the left of column signals firstly. When we block beams E3 and E3 in Fig. 2(b1), the reflection signal only includes the SNS resulting from ρ20(2) (see Appendix) which has one dip and one peak. The peak stands for the EIG and appears at the position of Δ1=Δ2 according to the generating term d20in the ρ10(3)(see Appendix). The dip appearing at the location of Δ1=Δ2+G2is the EIA caused by single photon term d10dressed by the term |G2|2/d20in theρ20(2). Also the position of the EIG and EIA moves with Δ1 changing .When one only block the beam E3in Fig. 2(b2), we can find that the peak becomes higher and dip becomes deeper compared with Fig. 2(b1) because of the optical pumping effect of the E3. Now we only block the laser beam E1in Fig. 2(b3), the EIG and EIA disappeared because the term G1=0 inρ20(2). In Fig. 2(b4), we open all the laser beams. One can find that the peak is higher than any cases illustrated in Fig. 2(b1)-2(b3) and thus a new peak is generated which does not belong to the SNS. If a peak appears in the case of scanning the dressing frequency detuningΔ2, the peak must be the enhancement of four wave mixing band gap signal (FWM BGS) satisfying the phase-matching kF = k1 + k3-k′3 which is actually SWM BGS [22]. The series expansion ofρ10(3) (see Appendix),ρ10(3)={-iG1G3G3[12(|G30|2/d30+|G2|2/d20)/d10]}/d30d102 shows us the equivalence between the enhancement of FWM BGS and SWM BGS, in which the last term iG1G3G3|G2|2/[(d10)3d30d20]is actually SWM BGS. The SWM BGS is generated byE1,E3,E3 and E2according to the condition of phase matching. And the peak is the sum of the SNS caused byρ20(2)and SWM BGS. We can see only one peak in Fig. 2(b4) since the SWM BGS fills up the dip caused by the EIA. Next, we consider the right column signal. The right column signal is the SNS resulted from theρ23(2). Also the right column signal locates about atΔ2=Δ3 whose position changes with Δ3 varying by considering the dressing term |G2|2/d23in theρ23(2). When we blockE3,E3 (Fig. 2 (b1)) or only block E3 (Fig. 2(b2)), the SNS disappears which results from the term G3=0in theρ23(2). When we open E3 and E3with blocking E1in Fig. 2(b3), one dip appears at Δ2=Δ3 due to the term |G2|2/d23 in theρ23(2). In Fig. 2(b4), we open all the laser beams, the dip is deeper compared with Fig. 2(b3) due to the increasing optical pumping effect of theE1.The corresponding fluorescence signals with the different laser beam blocked are also presented in Fig. 2(c). We analyze the left column signal first.When the beams E1 and E2 is turned on with E3and E3blocked in Fig. 2(c1), a peak described by ρ22D(4) (see Appendix) appears at Δ1=Δ2 whose position changes with Δ1 varying.Next when we openE1, E2 and E3 with only E3 blocked in Fig. 2(c2), it can be seen that the peak on the fluorescence is higher than the one in Fig. 2(c1).It is because that the nest dressing effect leads to the enhancement effect of E3on the peak according to the nest-dressing term|G2|2/(d10+|G30|2/d30) in theρ22D(4).When we only blockE1in Fig. 2(c3), the peak disappears according to the termG1=0in theρ22D(4). Physically, the source of fluorescence radiation is the excited transition of particles from the ground state, which disappeared with E1 blocked. In Fig. 2(c4), we open all laser beams. One can find that the peak becomes higher compared with the Fig. 2(c1) and Fig. 2(c2) because both E3and E3make the more enhancement effect on fluorescence. Next, we consider the right column signal. When beams E1 and E2 are turned on with E3and E3blocked (Fig. 2(c1)) or with E3 opened and only E3 blocked (Fig. 2(c2)), the peak caused by ρ22(4)disappears according to the term G3=0in theρ22(4). Next, we turn on beamsE2, E3and E3 with E1 blocked in Fig. 2(c3), there is a peak on the fluorescence located atΔ2=Δ3caused by the generating term d21in theρ22(4). And the location of peak changes with the Δ3varying. When we open all the laser beams in Fig. 2(c4), the peak becomes higher than the one in Fig. 2(c3) because of the enhancement effect of beam E1by considering the nest-dressing term |G2|2/(d13+|G1|2/d03) in theρ22(4).

 figure: Fig. 2

Fig. 2 Measured (a) probe transmission signal, (b) reflection signal, and (c) fluorescence versus Δ2 from 200 MHz to 550 MHz when different beams are blocked. (a1)- (c1) E3and E3 blocked, (a2)-(c2) E3blocked, (a3)-(c3) E1blocked, and (a4)-(c4) no beam blocked. Δ1 = −280 MHz and Δ3 = −450MHz.

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In following we concentrate on the signal intensity dependence on the power of laser beam by scanning Δ2in Fig. 3 . First, when the power of the beam E2(P2) changes from small to large, we arrange the experimental curves from bottom to top in Fig. 3(a1)-Fig. 3(c1). In Fig. 3(a1), the peak shows the enhancement of the probe transmission signal, which locates Δ2=Δ1decided by the term |G2|2/d20inρ10(1). When one changes P2 from small to large values, peaks become higher due to the increasing dressing effect of E2by considering the dressing term |G2|2/d20 in ρ10(1). The dip locating at Δ2=Δ3 represents the suppression of the probe transmission signal caused by the term |G2|2/d23inρ13(1) and dip is deeper also due to the stronger dressing effect ofE2according to the term |G2|2/d23inρ13(1) with P2 changes from small to large. Figure 3(b1) illustrates the competition between SWM BGS and SNS in the reflection signal channel. We analyze the right column signal first. The signal located at Δ2=Δ1is the sum of the SNS caused byρ20(2)and the SWM BGS. When we change P2 from small to large values, the signal switches from a dip to a peak and then the peak continues to become higher. It is because the SWM BGS fills up the dip caused by the EIA with the P2 increasing and then the peak will become higher since EIG and SWM BGS become larger with continuing to increase P2. For the left column signal, there is only a dip (EIA) locates at Δ2=Δ3G2caused by |G2|2/d23in theρ23(2)when the value of P2 is small. And with changing P2 from small to large, a peak caused by the term d23in ρ23(2) appears at the location of Δ2=Δ3 and becomes higher because of the classical effect of G2 in the numerator of ρ23(2). For the fluorescence in Fig. 3(c1), we consider the right column signal first. The dip represents that the second order fluorescence related to ρ11(2) is suppressed by the dressing effect of E2, which locates at Δ2=Δ1according to |G2|2/d20in ρ11(2). The peak is the fourth order fluorescence related toρ22D(4). In contrast, with P2 changes from small to large values, the dip becomes deeper and the peak becomes higher due to the increasing nest-dressing effect of E2 according to the nest-dressing term|G2|2/(d10+|G30|2/d30). Next we analyze the left column signal. The peak shows the fourth order fluorescence caused byρ22(4). When we change the P2 from small to large values, the peak becomes higher because the nest-dressing effect is increasing by considering the nest-term |G2|2/(d13+|G1|2/d03) in theρ22(4). The calculated probe transmission signal, reflection signal and fluorescence are displayed separately on Figs. 3(a2)-3(c2). Such theoretical calculations confirm our experimental analysis stated above.

 figure: Fig. 3

Fig. 3 For Fig. 3(a)-3(c), measured (a1) probe transmission signal, (b1) reflection signal and (c1) fluorescence versus Δ2, when we select five different discrete values of P2 as black (3.5 mW), red(2.4 mW), blue(1.5 mW), green(1.2 mW) and purple(0.7mW) and Δ3 = −110 MHz, Δ1 = −280 MHz. (a2), (b2) and (c2) are the theoretical calculations of (a1), (b1) and (c1), respectively. For Fig. 3(d)-3(f), measured (d1) probe transmission signal, (e1) reflection signal and (f1) fluorescence versus Δ2, when we select five different discrete values of P1 as black (10.05 mW), red(8.62 mW), blue(6.1 mW), green(3.83 mW) and purple(1.86 mW) and Δ3 = −410 MHz, Δ1 = −280 MHz. (d2), (e2) and (f2) are the theoretical calculations of (d1), (d1) and (f1), respectively.

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Next we concentrate on the signal intensity dependence on the power of the probe E1 (P1) in Fig. 3(d)-3(f). When the P1 changes from small to large, we arrange the experimental curves from bottom to top. In Fig. 3(d1), the peak caused by ρ10(1)locates at the position of Δ2=Δ1decided by the term |G2|2/d20 and the intensity of the peak increases with P1 increasing. The dip located at Δ2=Δ3 is caused by the term |G2|2/d23in ρ13(1)and it becomes deeper as P1 increases because of the increasing dressing effect of the term |G1|2/d03inρ13(1). We illustrate the reflection signal with the different P1 in Fig. 3(e1). There exist two columns of signals on the experimental curve and we consider the left column signal first. The signal located at Δ2=Δ1 stands for the sum of SWM BGS and SNS decided byρ20(2). As P1 increases, the peak becomes lower and then disappears and the dip continues to become deeper. It is because that the EIA in SNS is sensitive to the variation of P1 according to the dressing term |G1|2/Γ00 in ρ20(2) compared with SWM BGS. The right column signal is the SNS caused byρ23(2). When we change P1 from small to large values, the dip is deeper because of the dressing effect of the term |G1|2/d03inρ23(2). For fluorescence signal (Fig. 3(f1)), the left column signal locates at the position ofΔ2=Δ1.The intensity of peak which is mainly dependent on the beam E1 intensity according toρ22D(4) get greatly larger as P1 increases. The dip caused by the dressing term |G2|2/d20 in ρ11(2) appears when the value of P1 increases to a certain value. The dip becomes deeper with P1 increasing for the reason that G1 has the modification effect on the dressing effect of the term |G2|2/d20 inρ11(2). The right column signal is located atΔ2=Δ3according to ρ22(4) and the peak gets larger with P1 increasing, it is because that the nest-dressing effect in the term |G2|2/(d13+|G1|2/d03) of ρ22(4) becomes stronger. Especially, the calculated probe transmission signal, reflection signal and fluorescence are displayed separately on Figs. 3(d2)-3(f2). Such theoretical calculations confirm our experimental analysis stated above.

Finally, we observe the probe transmission signal, reflection signal and fluorescence under different detunings by scanning Δ2in Fig. 4 . First, when the coupling detuning Δ3 changes from small to large values, we arrange the experimental curves from bottom to top in Figs. 4(a1)-4(c1). For the probe transmission signal, the dip located atΔ2=Δ3 moves toward peak due to the term |G2|2/d23in ρ13(1)and the dip becomes smaller until invisible when we change Δ3to about the value ofΔ1. The peak locates at Δ2=Δ1according to the term|G2|2/d20inρ10(1). When one changes Δ3 to aboutΔ1, the intensity of the peak becomes lower due to the term |G30|2/d30 inρ10(1). The intensity of the peak will become stronger when Δ3 far awayΔ1. For the reflection signal (Fig. 4(b1)), the dip located at Δ2=Δ3 stands for the EIA caused by the term |G2|2/d23inρ23(2). And the position of EIA changes with the value of Δ3 varying. The dip will be deepest when Δ3 is near the value of Δ1 and it becomes shallower when Δ3 is far away from the value of Δ1because of the term |G1|2/d03inρ23(2). The peak located at Δ2=Δ1 is the sum of SWM BGS and SNS induced byρ20(2). The peak is smaller when we change Δ3 to about Δ1 because of the dressing effects of the term |G30|2/d30inρ20(2)and the term |G30|2/d30inρ10(5). When Δ3 is far away from the value ofΔ1, the peak becomes higher because the dressing effect of E3 decreases. Since the intensity of SNS is very small, the intensity of peak almost comes from SWM BGS. In Fig. 4(b1), we can modulate the intensity of SWM BGS through changingΔ3. Thus, the schematic diagram of the adjustable optical amplifier can be illustrated in Fig. 4(g) where we set the FWM BGS as input and SWM BGS is the enhancement of the FWM BGS. Further, SNS plays the modulation role which can control the amplification amplitude for FWM BGS through changing the detuningΔ3. Then SWM BGS modulated by SNS is the output of adjustable optical amplifier. In Fig. 4(c1), we observe the changes on the fluorescence when one changes the detuningΔ3. One peak located at Δ2=Δ3 is the fourth order fluorescence related to theρ22(4). Another peak which locates at Δ2=Δ1 is the fourth order fluorescence caused byρ22D(4). First, we consider the peak related to ρ22(4).When we change Δ3 from small to large values, the location of the peak is changing and the intensity of the peak is smaller because the increasing value of Δ3 makes the ρ22(4)(peak) smaller. Especially, whenΔ1=Δ3, the peak related to ρ22(4)overlaps with the peak caused by ρ22D(4). The peak is higher when we change Δ3 to about Δ1 and the peak becomes smaller when Δ3 is far away from the value of Δ1 due to the nest-dressing effect by considering the term |G2|2/(d10+|G30|2/d30) inρ22D(4). The calculated probe transmission signal, reflection signal and fluorescence are displayed separately on Figs. 4(a2)-4(c2). Such theoretical calculations confirm our experimental analysis stated above.

 figure: Fig. 4

Fig. 4 For Fig. 4(a)-4(c) measured (a1) probe transmission signal, (b1) reflection signal and (c1) fluorescence versus Δ2, when we select five different discrete values of Δ3 as black (−150MHz), red (−200MHz), blue (−280MHz), green (−350MHz) and purple (−450MHz) and Δ1 = −280 MHz. (a2), (b2) and (c2) are the theoretical calculations of (a1), (b1) and (c1), respectively. For Fig. 4(d)-4(f) measured (d1) probe transmission signal, (e1) reflection signal and (f1) fluorescence versus Δ2, when we select five different discrete values of Δ1 as black (−80MHz), red (−180MHz), blue (−280MHz), green (−300MHz) and purple (−380MHz) and Δ3 = −280 MHz. (d2), (e2) and (f2) are the theoretical calculations of (d1), (d1) and (f1), respectively. (g) the schematic diagram of the adjustable optical amplifier.

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Next, we analyze the changes on the reflection signal, the probe transmission signal and fluorescence when we set the different Δ1 values in Fig. 4(d1)-4(f1). Figure 4(d1) shows the influence of detuning Δ1on the probe transmission signal. The dip caused by theρ13(1)locates at Δ2=Δ3according to the term|G2|2/d23. The peak caused by theρ10(1)locates at Δ2=Δ1 denoting by the term |G2|2/d20 and the position of peak moves with the value of Δ1 changing. When we change the value of Δ1 from small to large, the intensity of peak is higher when the value of Δ1 is far away from Δ3 and peak becomes lower when Δ1 is nearΔ3. Especially, the intensity of the peak is smallest on the condition ofΔ1=Δ3. It is because of the dressing effect of the term |G30|2/d30 in ρ10(1). In Fig. 4(e1), we analyze the changes on the SWM BGS and SNS when the value of Δ1is different. We consider the dip located at the position of Δ2=Δ3first. The dip is the EIA caused byρ23(2). The dip becomes deeper in the case that the value of Δ1 is near Δ3 and the dip is shallower on the condition that Δ1 is far away from Δ3when we change Δ1 from small to big values. This is because the term |G1|2/d03 in ρ23(2)makes the intensity of dip changes. Now, we analyze the signal located atΔ2=Δ1. The signal is the sum of the SWM BGS and SNS caused by ρ20(2)and the position of the signal changes with the Δ1varying. WhenΔ3<Δ1, the signal is a peak which is the sum of SWM BGS and SNS and the intensity of peak is smaller with the Δ3increasing because the SWM BGS becomes smaller. Specially, whenΔ3=Δ1, the peak and the dip overlap. And then the signal becomes a dip which is the EIA because the SWM BGS disappeared in the case ofΔ3>Δ1. Figure 4(f1) illustrates the changes on the fluorescence when we set differentΔ1. One peak caused by ρ22(4)locates at Δ2=Δ3 and its position keeps fixed. Another peak caused by ρ22D(4) locates at Δ2=Δ1 and its position moves with Δ1 changing. When we change Δ1 from small to large values, the intensity of peak is lower on the condition of the value of Δ1 being far away from Δ3 and peak becomes higher when Δ1 is near Δ3. Especially, the intensity of the peak is highest on the condition ofΔ1=Δ3. It is because of the nest dressing effect of G30 by considering the term |G2|2/(d10+|G30|2/d30)inρ22D(4). Especially, the calculated probe transmission signal, reflection signal and fluorescence are displayed separately on Figs. 4(d2)-4(f2). Such theoretical calculations confirm our experimental analysis stated above.

4. Conclusion

In summary, the probe transmission signal, reflection signal, and fluorescence are compared for the first time in the case of scanning the dressing detuning. We experimentally and theoretically demonstrated the interplay between SNS and SWM BGS when we change the frequency detunings of the coupling and probe field as well as the powers of the probe and dressing field. We also observed the relation of the probe transmission signal and fluorescence. Such research could find its applications in adjustable optical amplifiers.

Appendix

According to the Liouville pathway [23] ρ00(0)ω1ρ10(1)andρ33(0)ω3ρ13(1), the first-order density matrix elementsρ10(1), ρ13(1)can be given as follows

ρ10(1)=iG1d10+|G30|2/d30+|G2|2/d20
ρ13(1)=iG3d13+|G1|2/d03+|G2|2/d23+|G30|2/Γ33
where |G30|2=|G3|2+|G3|2+2G3G3cos(2k3x), Gi=μiEi/is the Rabi frequency with transition dipole momentμi, d10=Γ10+iΔ1, d30=Γ30+iΔ1iΔ3, d20=Γ20+iΔ1+iΔ2, d13=iΔ3+Γ13, d03=i(Δ3Δ1)+Γ03, d23=i(Δ2+Δ3)+Γ23,frequency detuning Δi=Ωi-ωi (Ωi is the resonance frequency of the transition driven by Ei) and Γij is transverse relaxation rate between |iand|j. Via pathwaysρ00(0)ω1ρ10(1)ω2ρ20(2),ρ33(0)ω3ρ13(1)ω2ρ23(2), the second-order matrix elementsρ20(2),ρ23(2)can be described as follows
ρ20(2)=G1G2(d10+|G1|2/Γ00+|G2|2/d20+|G30|2/d30)*d20
ρ23(2)=G2G3(d13+|G1|2/d03+|G2|2/d23+|G30|2/Γ33)*d23
According to the pathwayρ00(0)ω1ρ10(1)(ω3)*ρ30(2)ω3ρ10(3), we can obtain the third-order matrix element ρ10(3)as follows
ρ10(3)=iG1G3G3(d10+|G30|2/d30+|G2|2/d20)2d30
Through the pathwayρ00(0)ω1ρ10(1)(ω3)*ρ30(2)ω3ρ10(3)ω2ρ20(4)(ω2)*ρ10(5), the fifth-order matrix element ρ10(5)can be obtained as follows

ρ10(5)=iG1G3G3|G2|2(d10+|G30|2/d30+|G2|2/d20)3d30d20

According to the relationε0χE=Nμρ, in which N, ε0 are the atom density and dielectric constant respectively, so the formulations of the linear and nonlinear susceptibilities can be obtained as follows:

χL=iNμ2ε01d10+|G30|2/d30+|G2|2/d20+iNμ2ε01d13+|G1|2/d03+|G30|2/Γ33+|G2|2/d23
χNL=iNμ2ε0[1(d10+|G30|2/d30+|G2|2/d20)2d301(d10+|G30|2/d30+|G2|2/d20)3d30d20]Nμ2ε01(d10+|G1|2/Γ00+|G2|2/d20+|G30|2/d30)*d20Nμ2ε01(d13+|G1|2/d03+|G2|2/d23+|G30|2/Γ33)*d23

In order to estimate the probe transmission signal and the reflection signal, we start from the nonlinear coupled wave equations [24,25 ],

E1(x)/x=αE1(x)+keiΔkxxEr(x)
Er(x)/x=αEr(x)+keiΔkxxE1(x)
Where E1(x) and Er(x) represent the probe transmission signal and reflection signal, respectively. α=(ω1/c)ImχL/2 is the attenuation of the field due to the absorption of the medium and k=i(ω1/c)χNL/2 is the gain due to the nonlinear susceptibility. χL, χNL are the zero order coefficients from Fourier expansion ofχL,χNL, respectively. Δkx={2(ω1cosθω3)+Re[χ(1)]ω1cosθ}/c is the phase mismatch magnitude, in which θ is the angle between probe E1 and E3. If the length of the sample in x direction is dx, by solving above equations, the reflection signal (R) and the probe transmission signal (T) are given as
R=|1keλ2+dxeλ2dxeλ2+dx(λ1++α)1eλ2dx(λ1+α)1|2
T=|e(λ1++λ1)dx(λ1λ1+)(λ1+α)eλ1dx(λ1++α)eλ1+dx|2
whereλ1±=iΔkx/2±[(αiΔkx/2)2k2]1/2,λ2±=λ1±+iΔkx.

For the fluorescence signals, with the only probe beam E1 turned on, the single-photon fluorescence R0 generates. We can describe the expression of ρ11(2)via the pathwayρ00(0)ω1ρ10(1)ω1*ρ11(2) asρ11(2)=|G1|2d10Γ11, the amplitude square of which is proportional to the intensity of R0. When we turn on the beams E2 and E3, the fluorescence R0 also dressed, via the pathwayρ00(0)ω1ρ+0(1)ω1*ρ++(2), the expression of ρ11(2)can be modified as

ρ11DD(2)=|G1|2(d10+|G30|2/d30+|G2|2/d20)Γ11
Next, in the two ladder type subsystems |0|1|2and|3|1|2, the two-photon fluorescence signals R1 and R2 generate separately. For signal R1 in|0|1|2 subsystem, through pathwayρ00(0)ω1ρ10(1)ω2ρ20(2)ω1*ρ21(3)ω2*ρ22(4)with the dressing effect of E3, the expression of density-matrix element ρ22D(4)can be obtained as
ρ22D(4)=|G1|2|G2|2Γ22d10d21[d20+|G1|2/d21+|G2|2/(d10+|G30|2/d30)]
whered21=Γ21+iΔ2, the amplitude square of which is proportional to the intensity of R1.

For signal R2 in|3|1|2subsystems, via the Liouville pathwayρ33(0)ω3ρ13(1)ω2ρ23(2)ω3*ρ21(3)ω2*ρ22(4), the expression of density-matrix element ρ22(4)can be described as

ρ22(4)=|G3|2|G2|2Γ22d13d21[d23+|G2|2/(d13+|G1|2/d03)+|G30|2/d21]
the amplitude square of which is proportional to the intensity of R2.

Acknowledgments

This work was supported by the 973 Program (2012CB921804), NSFC (61108017, 11474228), and KSTIT of Shaanxi Province (2014KCT-10), NSFC of Shaanxi Province (2014JZ020), FRFCU (2012jdhz05, xjj2012080), CPSF (2015T81030, 2014M560779) and Postdoctoral research project of Shaanxi Province.

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Figures (4)

Fig. 1
Fig. 1 (a) The setup of our experiment. (b) Inverted-Y type energy system. (c) Schematic of an electromagnetically induced grating formed by two coupling beams E3 and E′3 . (d) The single dressed energy level schematic diagrams and the calculated single dressed period energy levels. (e) The double dressed energy level schematic diagrams and the calculated double dressed periodic energy levels.
Fig. 2
Fig. 2 Measured (a) probe transmission signal, (b) reflection signal, and (c) fluorescence versus Δ2 from 200 MHz to 550 MHz when different beams are blocked. (a1)- (c1) E 3 and E 3 blocked, (a2)-(c2) E 3 blocked, (a3)-(c3) E 1 blocked, and (a4)-(c4) no beam blocked. Δ1 = −280 MHz and Δ3 = −450MHz.
Fig. 3
Fig. 3 For Fig. 3(a)-3(c), measured (a1) probe transmission signal, (b1) reflection signal and (c1) fluorescence versus Δ2, when we select five different discrete values of P2 as black (3.5 mW), red(2.4 mW), blue(1.5 mW), green(1.2 mW) and purple(0.7mW) and Δ3 = −110 MHz, Δ1 = −280 MHz. (a2), (b2) and (c2) are the theoretical calculations of (a1), (b1) and (c1), respectively. For Fig. 3(d)-3(f), measured (d1) probe transmission signal, (e1) reflection signal and (f1) fluorescence versus Δ2, when we select five different discrete values of P1 as black (10.05 mW), red(8.62 mW), blue(6.1 mW), green(3.83 mW) and purple(1.86 mW) and Δ3 = −410 MHz, Δ1 = −280 MHz. (d2), (e2) and (f2) are the theoretical calculations of (d1), (d1) and (f1), respectively.
Fig. 4
Fig. 4 For Fig. 4(a)-4(c) measured (a1) probe transmission signal, (b1) reflection signal and (c1) fluorescence versus Δ2, when we select five different discrete values of Δ3 as black (−150MHz), red (−200MHz), blue (−280MHz), green (−350MHz) and purple (−450MHz) and Δ1 = −280 MHz. (a2), (b2) and (c2) are the theoretical calculations of (a1), (b1) and (c1), respectively. For Fig. 4(d)-4(f) measured (d1) probe transmission signal, (e1) reflection signal and (f1) fluorescence versus Δ2, when we select five different discrete values of Δ1 as black (−80MHz), red (−180MHz), blue (−280MHz), green (−300MHz) and purple (−380MHz) and Δ3 = −280 MHz. (d2), (e2) and (f2) are the theoretical calculations of (d1), (d1) and (f1), respectively. (g) the schematic diagram of the adjustable optical amplifier.

Equations (15)

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ρ 10 ( 1 ) = i G 1 d 10 + | G 30 | 2 / d 30 + | G 2 | 2 / d 20
ρ 13 ( 1 ) = i G 3 d 13 + | G 1 | 2 / d 03 + | G 2 | 2 / d 23 + | G 30 | 2 / Γ 33
ρ 20 ( 2 ) = G 1 G 2 ( d 10 + | G 1 | 2 / Γ 00 + | G 2 | 2 / d 20 + | G 30 | 2 / d 30 ) * d 20
ρ 23 ( 2 ) = G 2 G 3 ( d 13 + | G 1 | 2 / d 03 + | G 2 | 2 / d 23 + | G 30 | 2 / Γ 33 ) * d 23
ρ 10 ( 3 ) = i G 1 G 3 G 3 ( d 10 + | G 30 | 2 / d 30 + | G 2 | 2 / d 20 ) 2 d 30
ρ 10 ( 5 ) = i G 1 G 3 G 3 | G 2 | 2 ( d 10 + | G 30 | 2 / d 30 + | G 2 | 2 / d 20 ) 3 d 30 d 20
χ L = i N μ 2 ε 0 1 d 10 + | G 30 | 2 / d 30 + | G 2 | 2 / d 20 + i N μ 2 ε 0 1 d 13 + | G 1 | 2 / d 03 + | G 30 | 2 / Γ 33 + | G 2 | 2 / d 23
χ N L = i N μ 2 ε 0 [ 1 ( d 10 + | G 30 | 2 / d 30 + | G 2 | 2 / d 20 ) 2 d 30 1 ( d 10 + | G 30 | 2 / d 30 + | G 2 | 2 / d 20 ) 3 d 30 d 20 ] N μ 2 ε 0 1 ( d 10 + | G 1 | 2 / Γ 00 + | G 2 | 2 / d 20 + | G 30 | 2 / d 30 ) * d 20 N μ 2 ε 0 1 ( d 13 + | G 1 | 2 / d 03 + | G 2 | 2 / d 23 + | G 30 | 2 / Γ 33 ) * d 23
E 1 ( x ) / x = α E 1 ( x ) + k e i Δ k x x E r ( x )
E r ( x ) / x = α E r ( x ) + k e i Δ k x x E 1 ( x )
R = | 1 k e λ 2 + d x e λ 2 d x e λ 2 + d x ( λ 1 + + α ) 1 e λ 2 d x ( λ 1 + α ) 1 | 2
T = | e ( λ 1 + + λ 1 ) d x ( λ 1 λ 1 + ) ( λ 1 + α ) e λ 1 d x ( λ 1 + + α ) e λ 1 + d x | 2
ρ 11 D D ( 2 ) = | G 1 | 2 ( d 10 + | G 30 | 2 / d 30 + | G 2 | 2 / d 20 ) Γ 11
ρ 22 D ( 4 ) = | G 1 | 2 | G 2 | 2 Γ 22 d 10 d 21 [ d 20 + | G 1 | 2 / d 21 + | G 2 | 2 / ( d 10 + | G 30 | 2 / d 30 ) ]
ρ 22 ( 4 ) = | G 3 | 2 | G 2 | 2 Γ 22 d 13 d 21 [ d 23 + | G 2 | 2 / ( d 13 + | G 1 | 2 / d 03 ) + | G 30 | 2 / d 21 ]
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