Abstract
For the first time, we experimentally and theoretically research about the second-order nonlinear signal (SNS) including electromagnetically induced absorbing (EIA) and electromagnetically induced gain (EIG), six wave mixing band gap signal (SWM BGS) resulting from photonic band gap structure in an inverted Y-type four level system with the electromagnetically induced grating. The interplay between the SNS and SWM BGS is illustrated clearly for the first time. When we change the frequency detuning to make the SWM BGS and SNS overlap, the SWM BGS is suppressed and the intensity of SNS is strongest near the resonance point. We can control the intensity of the SWM BGS and EIG caused by the classic effect through changing the power of coupling field. And the changes on the EIA generated by the quantum effect are obtained by changing the power of dressing field. Since the SWM BGS is the enhancement of the four wave mixing band gap signal (FWM BGS), when we set FWM BGS as the input and SNS as the modulation role to control the amplification amplitude for the FWM BGS in our scheme, the adjustable optical amplifier can be obtained.
© 2015 Optical Society of America
1. Introduction
Atomic coherence which can lead to a great many of significant physical phenomena is the result of interaction between light and materials. Recently, increasingly experimental researches are reported on the atomic coherence [1–3 ]. It is well-known that the six-wave mixing (SWM) is a nonlinear optical effect generated by lights with different frequencies and different quantum properties. In the nonlinear wave-mixing process, atomic coherence of the electromagnetically induced transparency (EIT) plays a critical role has been demonstrated experimentally and theoretically in recent researches [4–9 ]. Furthermore, the increasingly effect has been paid on the switch between EIT and electromagnetically induced absorption (EIA) [3,10 ]. In the EIT environment, SWM signal can transmit through the atomic medium and the fluorescence can be generated due to spontaneous emission [11–14 ]. And the EIT-based nonlinear schemes can be driven by traveling wave beams as well as by a standing wave (SW) which formed by the two same frequency counter propagating coupling fields [15,16 ]. Thus in an atomic system driven by two counter propagating coupling fields can obtain the large nonlinearity. It is reported that the electromagnetically induced grating [17,18 ] resulted from the interaction of the SW with the atomic coherent medium can possess photonic band gap (PBG) structure in a variety of interesting research results [19,20 ].
In this paper, the optical response of hot rubidium (85Rb) atoms driven by a SW is investigated in an inverted Y-type four level system and six wave mixing band gap signal (SWM BGS) and probe transmission signal are obtained firstly in the experiment. Especially, the two photon process including EIA and electromagnetically induced gain (EIG) are researched experimentally and theoretically for the first time. And we define the two photon process as the second-order nonlinear signals (SNS) in the paper. When we change the frequency detunings and the powers of the laser fields, the interplay between the SWM BGS and SNS as well as its application are also discussed for the first time in this paper. Furthermore, we also demonstrate the relation of the probe transmission signal and fluorescence in our research.
2. Experimental scheme
The experiment was completed in a rubidium atomic vapor cell of 85Rb. The energy levels 5S 1/2(F = 3) (|0>), 5S1/2(F = 2) (|3>), 5P3/2 (|1>) and 5D5/2 (|2>) compose a inverted-Y energy system as shown in Fig. 1(b) . Probe laser beam E1 (wavelength of 780.245 nm, frequency ω1 and wave vector k1) connects the transition 5S1/2 (F = 3) (|0>) to 5P3/2 (|1>). The laser beam E2 (wavelength of 775.978 nm, ω2, k2) drive an upper transition 5P3/2 (|1〉) to 5D5/2 (|2〉). A pair of coupling laser beams E3 (wavelength of 780.238 nm, ω3, k3) and E´3 (wavelength of 780.238 nm, ω´3, k´3) connect the transition 5S1/2(F = 2) (|3〉) to 5P3/2 (|1〉. The coupling field E3 and E´3 which propagate through 85Rb vapor in the opposite direction generate a standing wave , which results into an EIG. Furthermore EIG will lead to a PBG structure as shown in Fig. 1(c). In addition, the intensity of probe beam E1 is the only weak laser beam while other laser beams are strong. As illustrated on Fig. 1(a), the weak probe beam E1 propagates through the 85Rb vapors in the same direction of E´3 with a small angle between them. The dressing field E2 propagates in the opposite direction of E3 with a small angle between them. Due to the small angle between the probe beam E1 and the beam E´3, the geometry not only satisfies the phase-matching (kS = k1 + k2−k2 + k3-k′3) also provides a convenient spatial separation of the applied laser and generated signal beams. Thus we can detect the generated beams with highly directional [21]. The generated SWM BGS satisfies the phase-matching kS = k1 + k2−k2 + k3-k′3. Besides SWM BGS, there also exists SNS in the reflection signal channel as shown in Fig. 1(a). The reflection signal and the probe transmission signal are detected by a photodiode and avalanche photodiode detectors respectively. In addition, three fluorescence signals caused by spontaneous decay are measured. The second order fluorescence R0 and fourth order fluorescence R1, R2 are generated due to the spontaneous emission from and , respectively. Fluorescence signals are captured by another photodiode.
It is the essential to the generation of the PBG structure that the medium should have a periodic refractive index. In order to get the periodic refractive index, the susceptibility of the medium should be periodic by considering the relation of the refractive index with the susceptibility, i.e.,. Thus we must get the periodic energy level structure to generate the periodic susceptibility. Hence, the periodic energy levels can be obtained in Fig. 1(d)-1(e) by introducing periodic standing wave field. In Fig. 1(d), the level will be split into two dressed states. The two dressed states have the eigenvalues. And thevalues are also periodic along x because is periodic along x-axis. Thus we can obtain the periodic energy levels as shown in Fig. 1(e). When E2 is turn on, due to the second level dressing effect of E2, is further split into two dressed states. The two dressed states have the eigenvalueswith . Thus we also obtain the double dressed periodic energy levels as shown in Fig. 1(d)-1(e).
3. Results and discussions
First, we observe the probe transmission signal, reflection signal, and fluorescence when we block the different laser beam in case of scanning the frequency detuningin Fig. 2 . Figure 2(a) represents the changes on the probe transmission signal when different laser beams are blocked. When one block and in Fig. 2(a1), there is a peak on the probe transmission signal locating at the position of . And the peak stands for the enhancement of probe transmission signal caused by the term in (see Appendix). Next the beamis blocked in Fig. 2(a2), the peak is lower compared with the Fig. 2(a1) because of the strong cascade-dressing interaction between () and which leads to the suppression effect of on the peak by considering the cascade-dressing termin. When we block the beamin Fig. 2(a3), the peak disappeared because the term in. When all laser beams are opened in Fig. 2(a4), we can find that the peak on the probe transmission signal becomes lower than peaks in Fig. 2(a1) and Fig. 2(a2). The reason is that the cascade interaction which results in the suppression effect of on the peak plays a vital role on the intensity of peak. Figure 2(b) confirms the existence of SWM BGS and SNS in the reflection signal channel with the different laser beam blocked. Because the beam propagates in the opposite direction of in our experiment, the Doppler-free condition is satisfied in the subsystem and the experimental setup will be in the EIT environment. So the EIT-induced EIG will be generated in the EIT environment. Figure 2(b) has two columns of signals and we observe the left of column signals firstly. When we block beams and in Fig. 2(b1), the reflection signal only includes the SNS resulting from (see Appendix) which has one dip and one peak. The peak stands for the EIG and appears at the position of according to the generating term in the (see Appendix). The dip appearing at the location of is the EIA caused by single photon term dressed by the term in the. Also the position of the EIG and EIA moves with changing .When one only block the beam in Fig. 2(b2), we can find that the peak becomes higher and dip becomes deeper compared with Fig. 2(b1) because of the optical pumping effect of the . Now we only block the laser beam in Fig. 2(b3), the EIG and EIA disappeared because the term in. In Fig. 2(b4), we open all the laser beams. One can find that the peak is higher than any cases illustrated in Fig. 2(b1)-2(b3) and thus a new peak is generated which does not belong to the SNS. If a peak appears in the case of scanning the dressing frequency detuning, the peak must be the enhancement of four wave mixing band gap signal (FWM BGS) satisfying the phase-matching kF = k1 + k3-k′3 which is actually SWM BGS [22]. The series expansion of (see Appendix), shows us the equivalence between the enhancement of FWM BGS and SWM BGS, in which the last term is actually SWM BGS. The SWM BGS is generated by,, and according to the condition of phase matching. And the peak is the sum of the SNS caused byand SWM BGS. We can see only one peak in Fig. 2(b4) since the SWM BGS fills up the dip caused by the EIA. Next, we consider the right column signal. The right column signal is the SNS resulted from the. Also the right column signal locates about at whose position changes with varying by considering the dressing term in the. When we block, (Fig. 2 (b1)) or only block (Fig. 2(b2)), the SNS disappears which results from the term in the. When we open and with blocking in Fig. 2(b3), one dip appears at due to the term in the. In Fig. 2(b4), we open all the laser beams, the dip is deeper compared with Fig. 2(b3) due to the increasing optical pumping effect of the.The corresponding fluorescence signals with the different laser beam blocked are also presented in Fig. 2(c). We analyze the left column signal first.When the beams and is turned on with and blocked in Fig. 2(c1), a peak described by (see Appendix) appears at whose position changes with varying.Next when we open, and with only blocked in Fig. 2(c2), it can be seen that the peak on the fluorescence is higher than the one in Fig. 2(c1).It is because that the nest dressing effect leads to the enhancement effect of on the peak according to the nest-dressing term in the.When we only blockin Fig. 2(c3), the peak disappears according to the termin the. Physically, the source of fluorescence radiation is the excited transition of particles from the ground state, which disappeared with blocked. In Fig. 2(c4), we open all laser beams. One can find that the peak becomes higher compared with the Fig. 2(c1) and Fig. 2(c2) because both and make the more enhancement effect on fluorescence. Next, we consider the right column signal. When beams and are turned on with and blocked (Fig. 2(c1)) or with opened and only blocked (Fig. 2(c2)), the peak caused by disappears according to the term in the. Next, we turn on beams, and with blocked in Fig. 2(c3), there is a peak on the fluorescence located atcaused by the generating term in the. And the location of peak changes with the varying. When we open all the laser beams in Fig. 2(c4), the peak becomes higher than the one in Fig. 2(c3) because of the enhancement effect of beam by considering the nest-dressing term in the.
In following we concentrate on the signal intensity dependence on the power of laser beam by scanning in Fig. 3 . First, when the power of the beam (P2) changes from small to large, we arrange the experimental curves from bottom to top in Fig. 3(a1)-Fig. 3(c1). In Fig. 3(a1), the peak shows the enhancement of the probe transmission signal, which locates decided by the term in. When one changes P2 from small to large values, peaks become higher due to the increasing dressing effect of by considering the dressing term in . The dip locating at represents the suppression of the probe transmission signal caused by the term in and dip is deeper also due to the stronger dressing effect ofaccording to the term in with P2 changes from small to large. Figure 3(b1) illustrates the competition between SWM BGS and SNS in the reflection signal channel. We analyze the right column signal first. The signal located at is the sum of the SNS caused byand the SWM BGS. When we change P2 from small to large values, the signal switches from a dip to a peak and then the peak continues to become higher. It is because the SWM BGS fills up the dip caused by the EIA with the P2 increasing and then the peak will become higher since EIG and SWM BGS become larger with continuing to increase P2. For the left column signal, there is only a dip (EIA) locates at caused by in thewhen the value of P2 is small. And with changing P2 from small to large, a peak caused by the term in appears at the location of and becomes higher because of the classical effect of G2 in the numerator of . For the fluorescence in Fig. 3(c1), we consider the right column signal first. The dip represents that the second order fluorescence related to is suppressed by the dressing effect of E2, which locates at according to in . The peak is the fourth order fluorescence related to. In contrast, with P2 changes from small to large values, the dip becomes deeper and the peak becomes higher due to the increasing nest-dressing effect of E2 according to the nest-dressing term. Next we analyze the left column signal. The peak shows the fourth order fluorescence caused by. When we change the P2 from small to large values, the peak becomes higher because the nest-dressing effect is increasing by considering the nest-term in the. The calculated probe transmission signal, reflection signal and fluorescence are displayed separately on Figs. 3(a2)-3(c2). Such theoretical calculations confirm our experimental analysis stated above.
Next we concentrate on the signal intensity dependence on the power of the probe E1 (P1) in Fig. 3(d)-3(f). When the P1 changes from small to large, we arrange the experimental curves from bottom to top. In Fig. 3(d1), the peak caused by locates at the position of decided by the term and the intensity of the peak increases with P1 increasing. The dip located at is caused by the term in and it becomes deeper as P1 increases because of the increasing dressing effect of the term in. We illustrate the reflection signal with the different P1 in Fig. 3(e1). There exist two columns of signals on the experimental curve and we consider the left column signal first. The signal located at stands for the sum of SWM BGS and SNS decided by. As P1 increases, the peak becomes lower and then disappears and the dip continues to become deeper. It is because that the EIA in SNS is sensitive to the variation of P1 according to the dressing term in compared with SWM BGS. The right column signal is the SNS caused by. When we change P1 from small to large values, the dip is deeper because of the dressing effect of the term in. For fluorescence signal (Fig. 3(f1)), the left column signal locates at the position of.The intensity of peak which is mainly dependent on the beam E1 intensity according to get greatly larger as P1 increases. The dip caused by the dressing term in appears when the value of P1 increases to a certain value. The dip becomes deeper with P1 increasing for the reason that has the modification effect on the dressing effect of the term in. The right column signal is located ataccording to and the peak gets larger with P1 increasing, it is because that the nest-dressing effect in the term of becomes stronger. Especially, the calculated probe transmission signal, reflection signal and fluorescence are displayed separately on Figs. 3(d2)-3(f2). Such theoretical calculations confirm our experimental analysis stated above.
Finally, we observe the probe transmission signal, reflection signal and fluorescence under different detunings by scanning in Fig. 4 . First, when the coupling detuning changes from small to large values, we arrange the experimental curves from bottom to top in Figs. 4(a1)-4(c1). For the probe transmission signal, the dip located at moves toward peak due to the term in and the dip becomes smaller until invisible when we change to about the value of. The peak locates at according to the termin. When one changes to about, the intensity of the peak becomes lower due to the term in. The intensity of the peak will become stronger when far away. For the reflection signal (Fig. 4(b1)), the dip located at stands for the EIA caused by the term in. And the position of EIA changes with the value of varying. The dip will be deepest when is near the value of and it becomes shallower when is far away from the value of because of the term in. The peak located at is the sum of SWM BGS and SNS induced by. The peak is smaller when we change to about because of the dressing effects of the term inand the term in. When is far away from the value of, the peak becomes higher because the dressing effect of decreases. Since the intensity of SNS is very small, the intensity of peak almost comes from SWM BGS. In Fig. 4(b1), we can modulate the intensity of SWM BGS through changing. Thus, the schematic diagram of the adjustable optical amplifier can be illustrated in Fig. 4(g) where we set the FWM BGS as input and SWM BGS is the enhancement of the FWM BGS. Further, SNS plays the modulation role which can control the amplification amplitude for FWM BGS through changing the detuning. Then SWM BGS modulated by SNS is the output of adjustable optical amplifier. In Fig. 4(c1), we observe the changes on the fluorescence when one changes the detuning. One peak located at is the fourth order fluorescence related to the. Another peak which locates at is the fourth order fluorescence caused by. First, we consider the peak related to .When we change from small to large values, the location of the peak is changing and the intensity of the peak is smaller because the increasing value of makes the (peak) smaller. Especially, when, the peak related to overlaps with the peak caused by . The peak is higher when we change to about and the peak becomes smaller when is far away from the value of due to the nest-dressing effect by considering the term in. The calculated probe transmission signal, reflection signal and fluorescence are displayed separately on Figs. 4(a2)-4(c2). Such theoretical calculations confirm our experimental analysis stated above.
Next, we analyze the changes on the reflection signal, the probe transmission signal and fluorescence when we set the different values in Fig. 4(d1)-4(f1). Figure 4(d1) shows the influence of detuning on the probe transmission signal. The dip caused by thelocates at according to the term. The peak caused by thelocates at denoting by the term and the position of peak moves with the value of changing. When we change the value of from small to large, the intensity of peak is higher when the value of is far away from and peak becomes lower when is near. Especially, the intensity of the peak is smallest on the condition of. It is because of the dressing effect of the term in . In Fig. 4(e1), we analyze the changes on the SWM BGS and SNS when the value of is different. We consider the dip located at the position of first. The dip is the EIA caused by. The dip becomes deeper in the case that the value of is near and the dip is shallower on the condition that is far away from when we change from small to big values. This is because the term in makes the intensity of dip changes. Now, we analyze the signal located at. The signal is the sum of the SWM BGS and SNS caused by and the position of the signal changes with the varying. When, the signal is a peak which is the sum of SWM BGS and SNS and the intensity of peak is smaller with the increasing because the SWM BGS becomes smaller. Specially, when, the peak and the dip overlap. And then the signal becomes a dip which is the EIA because the SWM BGS disappeared in the case of. Figure 4(f1) illustrates the changes on the fluorescence when we set different. One peak caused by locates at and its position keeps fixed. Another peak caused by locates at and its position moves with changing. When we change from small to large values, the intensity of peak is lower on the condition of the value of being far away from and peak becomes higher when is near . Especially, the intensity of the peak is highest on the condition of. It is because of the nest dressing effect of G30 by considering the term in. Especially, the calculated probe transmission signal, reflection signal and fluorescence are displayed separately on Figs. 4(d2)-4(f2). Such theoretical calculations confirm our experimental analysis stated above.
4. Conclusion
In summary, the probe transmission signal, reflection signal, and fluorescence are compared for the first time in the case of scanning the dressing detuning. We experimentally and theoretically demonstrated the interplay between SNS and SWM BGS when we change the frequency detunings of the coupling and probe field as well as the powers of the probe and dressing field. We also observed the relation of the probe transmission signal and fluorescence. Such research could find its applications in adjustable optical amplifiers.
Appendix
According to the Liouville pathway [23] and, the first-order density matrix elements, can be given as follows
where , is the Rabi frequency with transition dipole moment, , , , , , ,frequency detuning ( is the resonance frequency of the transition driven by ) and is transverse relaxation rate between and. Via pathways,, the second-order matrix elements,can be described as follows According to the pathway, we can obtain the third-order matrix element as followsThrough the pathway, the fifth-order matrix element can be obtained as followsAccording to the relation, in which N, are the atom density and dielectric constant respectively, so the formulations of the linear and nonlinear susceptibilities can be obtained as follows:
In order to estimate the probe transmission signal and the reflection signal, we start from the nonlinear coupled wave equations [24,25 ],
Where E1(x) and Er(x) represent the probe transmission signal and reflection signal, respectively. is the attenuation of the field due to the absorption of the medium and is the gain due to the nonlinear susceptibility. , are the zero order coefficients from Fourier expansion of,, respectively. is the phase mismatch magnitude, in which is the angle between probe and . If the length of the sample in x direction is dx, by solving above equations, the reflection signal (R) and the probe transmission signal (T) are given as where,.For the fluorescence signals, with the only probe beam E1 turned on, the single-photon fluorescence R0 generates. We can describe the expression of via the pathway as, the amplitude square of which is proportional to the intensity of R0. When we turn on the beams E2 and E3, the fluorescence R0 also dressed, via the pathway, the expression of can be modified as
Next, in the two ladder type subsystems and, the two-photon fluorescence signals R1 and R2 generate separately. For signal R1 in subsystem, through pathwaywith the dressing effect of E3, the expression of density-matrix element can be obtained aswhere, the amplitude square of which is proportional to the intensity of R1.For signal R2 insubsystems, via the Liouville pathway, the expression of density-matrix element can be described as
the amplitude square of which is proportional to the intensity of R2.Acknowledgments
This work was supported by the 973 Program (2012CB921804), NSFC (61108017, 11474228), and KSTIT of Shaanxi Province (2014KCT-10), NSFC of Shaanxi Province (2014JZ020), FRFCU (2012jdhz05, xjj2012080), CPSF (2015T81030, 2014M560779) and Postdoctoral research project of Shaanxi Province.
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