金属基磷化物纳米材料制备与电催化应用研究进展

doi:10.11896/cldb.23080249

材料导报

2024, Vol. 38

Issue (8): 23080249-17 https://doi.org/10.11896/cldb.23080249

电化学能源材料与器件

金属基磷化物纳米材料制备与电催化应用研究进展

刘卉¹, 杨牛娃^1,2, 马梦圆^1,2, 田少囡^1,*, 张玉¹, 杨军^1,2,*

1 中国科学院过程工程研究所介科学与工程全国重点实验室,北京 100190
2 中国科学院大学材料科学与光电技术研究中心,北京 100049

Research Advances of Metal-based Phosphide Nanomaterials Toward Electrocatalytic Applications

LIU Hui¹, YANG Niuwa^1,2, MA Mengyuan^1,2, TIAN Shaonan^1,*, ZHANG Yu¹, YANG Jun^1,2,*

1 State Key Laboratory of Mesoscience and Engineering, Institute of Process Engineering, Chinese Academy of Sciences, Beijing 100190, China
2 Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China

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摘要处于纳米尺度的磷化物及其与贵金属构成的复合材料具有独特的物理和化学性质,在电催化领域有广泛应用。例如,在甲醇电催化氧化反应中,由于磷(P)比金属铂(Pt)或钯(Pd)等具有更大的电负性,金属原子的外层电子被P吸引而偏向P原子,从而间接提高了Pt或Pd 对CO类中间产物的耐受性;在电解水析氢反应中,P可以作为质子受体,增强H⁺在金属上的吸附,从而促进析氢反应;在电解水析氧反应中,金属基磷化物容易被氧化成氧化物和氢氧化物,从而形成氧化物/氢氧化物-磷化物界面,进一步促进析氧反应。纳米颗粒的催化性能很大程度上取决于催化剂的结构、组分、组分之间的相互作用以及活性位点的电子结构,因此,对金属基磷化物基纳米复合材料的这些性质进行合理调控是提升其电催化性能的关键。本文所综述的材料范围包含金属基磷化物本身及其与贵金属构成的纳米复合材料,首先概括介绍金属基磷化物基纳米复合材料的合成方法和表征技术,进而阐述如何利用复合材料中晶格应变和电子耦合等物理效应提升电催化活性和稳定性。最后,围绕金属基磷化物基纳米复合材料电催化性能进一步提升的问题,对其未来合成策略和发展进行展望。

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	刘卉
	杨牛娃
	马梦圆
	田少囡
	张玉
	杨军

关键词: 金属基磷化物纳米复合材料电催化甲醇氧化反应析氢反应析氧反应

Abstract: Nanometer sized metal phosphides and their nanocomposites with noble metals have unique physical/chemical properties that have been found wide applications in electrocatalysis. For instance, in methanol oxidation reaction, the shift of electron clouds from noble metals, e.g. Pt and Pd, to the phosphor (P) due to larger electronegativity of the latter would enhance thetolerance of noble metals for the CO-like interme-diates produced during methanol oxidation. Also, in hydrogen evolution reaction (HER) of electrocatalytic water splitting, the P element in the phosphide-based nanocomposites could strengthen the H⁺ adsorption by serving as proton acceptor, thus promoting the HER. In addition, in oxygen evolution reaction (OER), the metal phosphides could be easily transformed into metal oxides/hydroxides for forming metal phosphide-metal oxide/hydroxide interfaces that is capable to boost the OER. It is well known that the catalytic performance of a catalyst strongly depends on its structure, components and their interactions as well as the electronic configuration of the active sites. In this context, rational regulation of the above-mentioned properties of metal phosphide-based nanocomposites is of necessity to improve their electrocatalytic performance. It is noteworthy that the materials in this review include metal phosphides and their nanocomposites with different nobles. We would firstly introduce the synthesis and characterization of metal phosphide-based nanocomposites, and subsequently, we focus on reviewing recent advances and challenges in making use of the lattice strain effect and electronic coupling effect to boost the performance of metal phosphide-based nanocomposites in typical electrochemical reactions. Eventually, regarding further improvement in elecrtocatalytic performance, we make some perspectives on the future synthetic strategies and development of the metal phosphide-based nanocomposites.

Key words: metal-based phosphide nanocomposite electrocatalysis methanol oxidation reaction hydrogen evolution reaction oxygen evolution reaction

出版日期: 2024-04-25 发布日期: 2024-04-28

ZTFLH:

O646

基金资助: 国家自然科学基金(22075290;22272179);北京自然科学基金(Z200012)

通讯作者: *田少囡,2017年博士毕业于北京工业大学,中国科学院过程工程研究所高级工程师,过程所模块化平台公共仪器中心主任,硕士研究生导师,入选中国科学院稳定支持青年团队计划;作为课题负责人致力于含重金属有机固废循环利用技术研发和环境风险分析评价等相关研究工作。sntian@ipe.ac.cn
杨军,中国科学院过程工程研究所研究员,中国科学院大学材料科学与光电技术学院岗位教授、博士研究生导师。2006年于新加坡国立大学获得博士学位,2006—2007年先后在波士顿大学、多伦多大学进行博士后研究,2007—2010年在新加坡生物工程与纳米技术研究院从事研究工作,2010年回国工作,创建能源转化与环境净化材料课题组,主要从事贵金属基异质结构纳米材料的构筑及其在能源转化和环境净化方面的应用研究。jyang@ipe.ac.cn

作者简介: 刘卉,中国科学院过程工程研究所副研究员、硕士研究生导师。2010年于北京科技大学获得硕士学位,2014年于中国科学院过程工程研究所获得博士学位,主要研究方向是新型纳米复合材料的合成以及用于能量转换和环境修复。

引用本文:

刘卉, 杨牛娃, 马梦圆, 田少囡, 张玉, 杨军. 金属基磷化物纳米材料制备与电催化应用研究进展[J]. 材料导报, 2024, 38(8): 23080249-17.
LIU Hui, YANG Niuwa, MA Mengyuan, TIAN Shaonan, ZHANG Yu, YANG Jun. Research Advances of Metal-based Phosphide Nanomaterials Toward Electrocatalytic Applications. Materials Reports, 2024, 38(8): 23080249-17.

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http://www.mater-rep.com/CN/10.11896/cldb.23080249 或 http://www.mater-rep.com/CN/Y2024/V38/I8/23080249

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