Facile self-propagated carbonization synthesis of phosphorus-doped carbon-based catalysts for partial oxidation and hydrogenation

Huan Wang; Weitao Wang; Xulu Jiang; Zhen-Hong He; Kuan Wang; Yang Yang; Zhao-Tie Liu; Buxing Han

doi:10.1039/D2GC01359B

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Facile self-propagated carbonization synthesis of phosphorus-doped carbon-based catalysts for partial oxidation and hydrogenation†

Huan Wang,^a Weitao Wang,

*^a Xulu Jiang,^a Zhen-Hong He,

^a Kuan Wang,

^a Yang Yang,

^a Zhao-Tie Liu

*^ab and Buxing Han

*^c

Author affiliations

* Corresponding authors

^a College of Chemistry & Chemical Engineering, Shaanxi Key Laboratory of Chemical Additives for Industry, Shaanxi University of Science & Technology, Xi'an, Shaanxi, China
E-mail: wangweitao@sust.edu.cn, ztliu@snnu.edu.cn

^b School of Chemistry & Chemical Engineering, Shaanxi Normal University, Xi'an, Shaanxi, China

^c Beijing National Laboratory for Molecular Sciences (BNLMS), Centre for Molecular Science, Institute of Chemistry, Chinese Academy of Sciences, Beijing 100190, China
E-mail: Hanbx@iccas.ac.cn

Abstract

In this work, a fast and self-propagated carbonization (SPC) method to prepare phosphorus-doped carbon (PDC) and hybrid materials is proposed. PdZr/PDC prepared by the SPC method has good catalytic performance for both partial oxidation of benzyl alcohol to benzaldehyde and partial hydrogenation of phenol to cyclohexanone. The method has some obvious advantages, such as being simple and clean, and can be used easily for the large-scale preparation of the materials.

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DOI: https://doi.org/10.1039/D2GC01359B
Article type: Communication
Submitted: 09 Apr 2022
Accepted: 18 Jul 2022
First published: 19 Jul 2022

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Green Chem., 2022,24, 6108-6112

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Facile self-propagated carbonization synthesis of phosphorus-doped carbon-based catalysts for partial oxidation and hydrogenation

H. Wang, W. Wang, X. Jiang, Z. He, K. Wang, Y. Yang, Z. Liu and B. Han, Green Chem., 2022, 24, 6108 DOI: 10.1039/D2GC01359B

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Green Chemistry

Facile self-propagated carbonization synthesis of phosphorus-doped carbon-based catalysts for partial oxidation and hydrogenation†

Abstract

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Facile self-propagated carbonization synthesis of phosphorus-doped carbon-based catalysts for partial oxidation and hydrogenation

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