In recent years, the "Taiwan Coffee" has become a hot topic and many farmers have invested in coffee growth. Because the production costs of coffee in Taiwan are relatively high, the development of coffee industry in Taiwan must be alliance with leisure agriculture. Through understanding the development of the Taiwan coffee industry and developing the evaluation criteria framework, the purpose of this study is to investigate the location choice of Taiwan coffee industry in alliance with leisure agriculture. The expert questionnaire survey and Analysis Hierarchy Process (AHP) will be adopted in this study. In the evaluation criteria framework, natural conditions, production factors, marketing factors, and environmental resources are selected as criteria. Guosing Township at Nantou County, Gukeng Township at Yunlin County, Meishan Township at Chiayi County, Dongshan Township at Tainan County are selected as alternatives. The results of this study show that the priority order of criteria is: natural conditions, marketing factors, and environmental resources, and production factors. The top five priorities of sub-criteria are: production-marketing organization, climate, water and soil conservation, close to the market, and traffic convenience. The priority order of four alternatives to develop Taiwan coffee industry in alliance with leisure agriculture is: Gukeng Township, Dongshan Township, Meishan, and Guosing Township. The strategies to develop coffee industry at Gukeng Township will be suggested to enforce the advantages of production-marketing organization, close to the market, traffic convenience, fitness of tourism resources nearby, and baking technology.