Published March 1, 2019 | Version v1
Journal article Open

Strain-tunable magnetism at oxide domain walls

  • 1. Technical University of Denmark
  • 2. Bar-Ilan University
  • 3. Stanford University, Zhejiang University
  • 4. Stanford University

Description

Applying stress to a ferroelastic material results in a nonlinear strain response as domains of different orientations mechanically switch. The ability to write, erase and move domain walls between such ferroelastic domains suggests a method for making nanoelectronics where the domain wall is the device. However, little is known about the magnetic properties of such domain
walls. A fascinating model system is SrTiO3, where the ferroelastic domain walls display strain-tunable polarity and enhanced
conductivity. Here, we reveal a long-range magnetic order with modulations along the ferroelastic domain walls in SrTiO3 and
SrTiO3-based heterointerfaces, which manifests itself as a striped pattern in scanning superconducting quantum interference
device maps of the magnetic landscape. In conducting interfaces, the magnetism is coupled to itinerant electrons with clear signatures in magnetotransport measurements. The magnetic state is also coupled dynamically to the lattice and can be reversibly
tuned by applying local external forces. This study raises the possibility of designing nanoscale devices based on domain walls
where strain-tunable ferroelectric, ferroelastic and ferromagnetic orders may coexist.
 

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