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Title: Radioactive rare gases and tritium in the sample return container, and the $sup 37$Ar and $sup 39$Ar depth profile in the Apollo 16 drill stem

Technical Report ·
DOI:https://doi.org/10.2172/4333257· OSTI ID:4333257

The gas was extracted from the sample return container from the Apollo 16 and 17 missions by adsorption on charcoal and activated vanadium metal. The hydrogen, argon, and radon were separated and counted to give the tritium, /sup 37/Ar, /suyp 39/Ar, and /sup 222 /Rn activities. The tritium and argon activities observed could be explained by diffusive losses of these gases from the fine material in the container. There was no excess tritium present in the Apollo 17 containers that could be attributed to solar tritons remaining from the intense flare of August 4, 1972. The /sup 222/Rn observed in the sample return container was interpreted as an emanation product from lunar fines and an emanation yield of 1 x 10/sup -4/ was calculated. This yield is consistent with the low radon content observed in the lunar atmosphere. The tritium, sup 37/Ar, / sup 39/Ar, and /sup 222/Rn activities and the K, Ca, Ti, Fe, and Mn contents were measured on a set of samples from the Apollo 16 deep drill stem at depths from 83 to 343 g/cm/sup 2/. The /sup 37/Ar and /sup 39/Ar activities combined with similar measurements at more shallow depth by Fireman and associates (SAO) give the complete activity proflle in the lunar regolith. Since /sup 37/Ar is produced mainly by the /sup 40/Ca(n, alpha )/su p 37/Ar reaction it is possible to determine the neutron production rate in the regolith as a function of the depth. The /sup 222/Rn extracted from the samples by vacuum melting was found to be lower than expected in some samples based upon their uranium contents. The hydrogen and helium contents of the drill stem samples were measured and found to be relatively uniform with depth in contrast to similar measurements on Apollo 15 and 17 drill stems. The H/He atom ratio was higher than the accepted solar-wind value by a factor of two, possibly due to water contamination. (auth)

Research Organization:
Brookhaven National Laboratory (BNL), Upton, NY (United States)
NSA Number:
NSA-29-025062
OSTI ID:
4333257
Report Number(s):
BNL-18580
Resource Relation:
Other Information: Orig. Receipt Date: 30-JUN-74
Country of Publication:
United States
Language:
English