Skip to main content
Log in

Buildup characteristics of roof pollutants in the Shanghai urban area, China

  • Published:
Journal of Zhejiang University-SCIENCE A Aims and scope Submit manuscript

Abstract

The buildup of roof pollutants in an urban area of Shanghai, China was investigated by conducting 16 experiments between November 2007 and October 2008. Concentrations of Cu, Zn and Cd in runoff from three types of roof (concrete, aluminum and glass) exceeded USEPA National Recommended Water Quality Criteria. The solid/liquid partition of the selected metal elements was consistent for the three roof types: Al, Fe, Zn and Pb were present mainly in the particle-bound form, while the total loading of Cd was nearly 100% in the dissolved form. Atmospheric dry precipitation accounted for most of all pollutant loadings for all roof types, while roof material made only a minor contribution to the loadings. All pollutant accumulation rates except for COD showed a seasonal trend with peaks in spring (March∼May) and winter (December∼February) and troughs in summer (June∼August) and autumn (September∼November). Our results showed that a linear equation is the most reliable of commonly used buildup models to simulate the total phosphorus (TP) and total suspended solids (TSS) buildup processes on aluminum roofs and glass roofs. This study provided novel information about roof runoff in Shanghai, China, in terms of pollution status, pollution source and pollutant buildup processes, thereby aiding in rainwater utilization and non-point pollution control.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Similar content being viewed by others

References

  • Akan, A.O., Schafran, G.C., Pommerenk, P., Harrell, L.J., 2000. Modeling storm-water runoff quantity and quality from marine drydocks. Journal of Environmental Engineering, 126(1):5–11. [doi:10.1061/(ASCE)0733-9372(2000)126:1(5)]

    Article  Google Scholar 

  • APHA (American Public Health Association), 1998. Standard Methods for the Examination of Water and Wastewater (20th Ed.). Washington, D.C.

  • Brezonik, P.L., Stadelmann, T.H., 2002. Analysis and predictive models of stormwater runoff volumes, loads, and pollutant concentrations from watersheds in the Twin Cities metropolitan area, Minnesota, USA. Water Research, 36(7):1743–1757. [doi:10.1016/S0043-1354(01)00375-X]

    Article  Google Scholar 

  • Bucheli, T.D., Müller, S.R., Voegelin, A., Schwarzenbach, R.P., 1998a. Bituminous roof sealing membranes as major sources of the herbicide (R, S)-mecoprop in roof runoff waters: potential contamination of groundwater and surface waters. Environmental Science & Technology, 32(22):3465–3471. [doi:10.1021/es980318f]

    Article  Google Scholar 

  • Bucheli, T.D., Müller, S.R., Heberle, S., Schwarzenbach, R.P., 1998b. Occurrence and behavior of pesticides in rainwater, roof runoff, and artificial stormwater infiltration. Environmental Science & Technology, 32(22):3457–3464. [doi:10.1021/es980317n]

    Article  Google Scholar 

  • Chang, M., McBroom, M.W., Beasley, R.S., 2004. Roofing as a source of nonpoint water pollution. Journal of Environmental Management, 73(4):307–315. [doi:10.1016/j.jenvman.2004.06.014]

    Article  Google Scholar 

  • Chen, J., Adams, B.J., 2006. Analytical urban storm water quality models based on pollutant buildup and washoff processes. Journal of Environmental Engineering, 132(10):1314–1330. [doi:10.1061/(ASCE)0733-9372(2006)132:10(1314)]

    Article  Google Scholar 

  • Clark, S.E., Burian, S., Pitt, R., Field, R., 2007. Urban wet-weather flows. Water Environment Research, 79(10):1166–1227. [doi:10.2175/106143007X218386]

    Article  Google Scholar 

  • Cristina, C.M., Sansalone, J.J., 2000. Kinematic wave model of urban pavement rainfall-runoff subject to traffic loadings. Journal of Environmental Engineering, 126(7):629–636. [doi:10.1061/(ASCE)0733-9372(2003)129:7(629)]

    Article  Google Scholar 

  • Deletic, A., Orr, D.W., 2005. Pollution buildup on road surfaces. Journal of Environmental Engineering, 131(1):49–59. [doi:10.1061/(ASCE)0733-9372(2005)131:1(49)]

    Article  Google Scholar 

  • Förster, J., 1996. Patterns of roof runoff contamination and their potential implication on practice and regulation of treatment and local infiltration. Water Science & Technology, 33(6):39–48. [doi:10.1016/0273-1223(96)00329-0]

    Article  Google Scholar 

  • Förster, J., 1998. The influence of location and season on the concentrations of macroions and organic trace pollutants in roof runoff. Water Science & Technology, 38(10):83–90. [doi:10.1016/S0273-1223(98)00736-7]

    Article  Google Scholar 

  • Förster, J., 1999. Variability of roof runoff quality. Water Science & Technology, 39(5):137–144. [doi:10.1016/S0273-1223(99)00095-5]

    Article  Google Scholar 

  • Huang, X., Olmez, I., Aras, N.K., Gordon, G.E., 1994. Emissions of trace elements from motor vehicles: potential marker elements and source composition profile. Atmospheric Environment, 28(8):1385–1931. [doi:10.1016/1352-2310(94)90201-1]

    Article  Google Scholar 

  • Kang, J.H., Kayhanian, M., Stenstrom, M.K., 2006. Implication of a kinematic wave model for first flush treatment design. Water Research, 40(20):3820–3830. [doi:10.1016/j.watres.2006.09.007]

    Article  Google Scholar 

  • Kayhanian, M., Suverkropp, C., Rubyb, A., Tsay, K., 2007. Characterization and prediction of highway runoff constituent event mean concentration. Journal of Environmental Management, 85(2):279–295. [doi:10.1016/j.jenvman.2006.09.024]

    Article  Google Scholar 

  • Kim, L.H., Kayhanian, M., Zoh, K.D., Stenstrom, M.K., 2005. Modeling of highway stormwater runoff. Science of the Total Environment, 348(1–3):1–18. [doi:10.1016/j.scitotenv.2004.12.063]

    Article  Google Scholar 

  • Kim, L.H., Zoh, K.D., Jeong, S.M., Kayhanian, M., Stenstrom, M.K., 2006. Estimating pollutant mass accumulation on highways during dry periods. Journal of Environmental Engineering, 132(9):985–993. [doi:10.1061/(ASCE)0733-9372(2006)132:9(985)]

    Article  Google Scholar 

  • Lau, S.L., Stenstrom, M.K., 2005. Metals and PAHs adsorbed to street particles. Water Research, 39(17):4083–4092. [doi:10.1016/j.watres.2005.08.002]

    Article  Google Scholar 

  • Ning, J., 2005. Study on Rainstorm Intensity Formula for Short Duration and Design Hyetograph of Shanghai. MS Thesis, Department of Environmental Engineering, Tongji University, Shanghai, China (in Chinese).

    Google Scholar 

  • Sansalone, J.J., Buchberger, S.G., 1997. Partitioning and first flush of metals in urban roadway storm water. Journal of Environmental Engineering, 123(2):134–143. [doi:10.1061/(ASCE)0733-9372(1997)123:2(134)]

    Article  Google Scholar 

  • Shu, J., Dearing, J.A., Morse, A.P., Yu, L., Yuan, N., 2001. Determining the sources of atmospheric particles in Shanghai, China, from magnetic and geochemical properties. Atmospheric Environment, 35(15):2615–2625. [doi:10.1016/S1352-2310(00)00454-4]

    Article  Google Scholar 

  • Soonthornnonda, P., Christensen, E.R., Liu, Y., Li, J., 2008. A washoff model for stormwater pollutants. Science of the Total Environment, 402(2–3):248–256. [doi:10.1016/j.scitotenv.2008.04.036]

    Article  Google Scholar 

  • Tomanovic, A., Maksimovic, C., 1996. Improved modeling of suspended solids discharge from asphalt surface during storm event. Water Science & Technology, 33(4-5):363–369. [doi:10.1016/0273-1223(96)00253-3]

    Article  Google Scholar 

  • USEPA (US Environmental Protection Agency), 2006. National Recommended Water Quality Criteria-Correction. Office of Water EPA 822-B-00-021, Washington, D.C.

  • van Metre, P.C.M., Mahler, B.J., 2003. The contribution of particles washed from rooftops to contamination loading to urban streams. Chemosphere, 52(10):1727–1741. [doi:10.1016/S0045-6535(03)00454-5]

    Article  Google Scholar 

  • Yan, M., Kahawita, R., 2000. Modelling the fate of pollutant in overland flow. Water Research, 34(13):3335–3344. [doi:10.1016/S0043-1354(00)00053-1]

    Article  Google Scholar 

  • Zhang, J., Cheng, Z., Wang, W., 1998. Source apportionment on fine particles in atmosphere in Beijing. Acta Scientiae Circumstantiae, 18:62–67.

    Google Scholar 

  • Zobrist, J., Müller, S.R., Ammann, A., Bucheli, T.D., Mottier, V., Ochs, M., Schoenenberger, R., Eugster, J., Boller, M., 2000. Quality of roof runoff for groundwater infiltration. Water Research, 34(5):1455–1462. [doi:10.1016/S0043-1354(99)00290-0]

    Article  Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Tian Li.

Additional information

Project supported by the National Key Technology R&D Program of China (No. 2006BAK13B04), and the Expo Shanghai Sci-Tech Program of Science and Technology Commission of Shanghai (No. 06dz05808), China

Rights and permissions

Reprints and permissions

About this article

Cite this article

Wang, B., Li, T. Buildup characteristics of roof pollutants in the Shanghai urban area, China. J. Zhejiang Univ. Sci. A 10, 1374–1382 (2009). https://doi.org/10.1631/jzus.A0920019

Download citation

  • Received:

  • Revised:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1631/jzus.A0920019

Key words

CLC number

Navigation