Abstract
We present femtosecond time-resolved transient absorption data taken on polydiacetylene-pTS single crystals over the entire wavelength region of exciton resonance. Observed optical changes are accounted for by a model which predicts quantitatively the large resonant and nonresonant optical nonlinearities.
Similar content being viewed by others
References
S. Schmitt-Rink, D. S. Chemla, and D. A. B. Miller, Phys. Rev. B 32, 6601 (1985).
B. I. Greene, J. Orenstein, R. R. Millard, and L. R. Williams, Phys. Rev. Lett. 58, 2750 (1987).
B. I. Greene, J. Orenstein, R. R. Millard, and L. R. Williams, Chem. Phys. Lett. 139, 381 (1987).
M. Thakur and S. Meyler, Macromolecules 18, 2341 (1985).
M. Pope and C. E. Swenberg, “Electronic Processes in Organic Crystals” (Oxford Univ. Press, New York, 1982).
S. Suhai, J. Chem. Phys. 85, 611 (1986).
F. Wudl and S. P. Bitler, J. Am. Chem. Soc. 108, 4685 (1986).
V. M. Agranovich and M. D. Galanin, “Electronic Energy Transfer in Condensed Matter” (North-Holland, Amsterdam, 1982).
B. I. Greene, J. Orenstein, S. Schmitt-Rink, M. Thakur and D. H. Rapkine, in preparation.
Author information
Authors and Affiliations
Rights and permissions
About this article
Cite this article
Greene, B.I., Orenstein, J., Thakur, M. et al. Nonlinear Optical Response of Excitons Confined to one Dimension. MRS Online Proceedings Library 109, 159–162 (1987). https://doi.org/10.1557/PROC-109-159
Published:
Issue Date:
DOI: https://doi.org/10.1557/PROC-109-159