Experimental violation of the local realism for four-qubit Dicke state

Dicke state is an widely used type of multi-particle entangled state in quantum information. However, very few works have been done on its nonlocality. Here we prepare a four-photon symmetric Dicke state, whose fidelity is as high as 0 .904± 0.004, and devise a simple Bell-type inequality to demonstrate that it violates the local realism with 12 standard deviation. © 2015 Optical Society of America OCIS codes: (270.0270) Quantum optics; (270.4180) Multiphoton processes; (270.5585) Quantum information and processing. References and links 1. A. K. Ekert, “Quantum cryptography based on Bell’s theorem,” Phys. Rev. Lett. 67, 661 (1991). 2. V. Scarani and N. Gisin, “Quantum communication between N partners and Bell’s inequalities,” Phys. Rev. Lett. 87. 117901 (2001). 3. A. Sen, U. Sen and M.̇ Zukowski, “Unified criterion for security of secret sharing in terms of violation of Bell inequalities,” Phys. Rev. A68, 032309 (2003). 4. Č. Brukner, M.Żukowski, J. W. Pan, and A. Zeilinger, “Bell’s inequalities and quantum communication complexity,” Phys. Rev. Lett. 92, 127901 (2004). 5. S. Pironio, A. Acín, S. Massar, A. Boyer de la Giroday, D. N. Matsukevich, P. Maunz, S. Olmschenk, D. Hayes, L. Luo, T. A. Manning and C. Monroe, “Random numbers certified by Bell’s theorem,” Nature 464, 1021–1024 (2010). 6. J. F. Clauser, M. A. Horne, A. Shimony and R. A. Holt, “Proposed experiment to test local hidden-variable theories,” Phys. Rev. Lett. 23, 880 (1969). 7. R. F. Werner and M. M. Wolf, “All-multipartite Bell-correlation inequalities for two dichotomic observables per site,” Phys. Rev. A64, 032112 (2001). 8. H. Weinfurter and M.̇Zukowski, “Four-photon entanglement from down-conversion,” Phys. Rev. A 64, 010102 (2001). 9. M. Żukowski and C. Brukner, “Bell’s theorem for general N-qubit states,” Phys. Rev. Lett. 88, 210401 (2002). 10. Y. C. Wu, P. Badziag and M.̇ Zukowski, “Clauser-Horne-Shimony-Holt-type Bell inequalities involving a party with two or three local binary settings,” Phys. Rev. A 79, 022110 (2009). 11. N. D. Mermin, “Extreme quantum entanglement in a superposition of macroscopically distinct states,” Phys. Rev. Lett. 65, 1838 (1990). 12. M. Ardehali, “Bell inequalities with a magnitude of violation that grows exponentially with the number of particles,” Phys. Rev. A46, 5375 (1992). 13. A. V. Belinskii and D. N. Klyshko, “Interference of light and Bell’s theorem,” Phys. Usp. 36, 653 (1993). 14. J. Tura, R. Augusiak, A. B. Sainz, T. Vértesi, M. Lewenstein, A. Acín, “Detecting nonlocality in many-body quantum states,” Science 344, 1256–1258 (2014). 15. J. Tura, R. Augusiak, A. B. Sainz, B. Lücke, C. Klempt, M. Lewenstein, A. Acín, “Nonlocality in many-body quantum systems detected with two-body correlators,” Ann. Phys. 362, 370–423 (2015). 16. I. Pitowsky, “Quantum probability, quantum logic,” Lecture Notes in Physics (Springer-Verlag, 1989), Vol. 321. #247024 Received 13 Aug 2015; revised 6 Nov 2015; accepted 10 Nov 2015; published 13 Nov 2015 © 2015 OSA 16 Nov 2015 | Vol. 23, No. 23 | DOI:10.1364/OE.23.030491 | OPTICS EXPRESS 30491 17. Y. C. Wu, M.Żukowski, J. L. Chen, and G. C. Guo, “Compact Bell inequalities for multipartite experiments,” Phys. Rev. A88, 022126 (2013). 18. R. H. Dicke, “Coherence in spontaneous radiation processes,” Phys. Rev. 93, 99 (1954). 19. N. Kiesel, C. Schmid, G. Tóth, E. Solano, and H. Weinfurter, “Experimental observation of four-photon entangled Dicke state with high fidelity,” Phys. Rev. Lett. 98, 063604 (2007). 20. R. Krischek, C. Schwemmer, W. Wieczorek, H. Weinfurter, P. Hyllus, L. Pezzé and A. Smerzi, “Useful multiparticle entanglement and sub-shot-noise sensitivity in experimental phase estimation,” Phys. Rev. Lett. 107, 080504 (2011). 21. P. Hyllus, W. Laskowski, R. Krischek, C. Schwemmer, W. Wieczorek, H. Weinfurter, L. Pezzé, and A. Smerzi, “Fisher information and multiparticle entanglement,” Phys. Rev. A 85, 022324 (2012). 22. L. M. Duan, “Entanglement detection in the vicinity of arbitrary Dicke states,” Phys. Rev. Lett. 107, 180502 (2012). 23. W. Wieczorek, R. Krischek, N. Kiesel, P. Michelberger, G. Tóth, and H. Weinfurter, “Experimental entanglement of a six-photon symmetric Dicke state,” Phys. Rev. Lett. 103, 020504 (2009). 24. R. Prevedel, G. Cronenberg, M. S. Tame, M. Paternostro, P. Walther, M. S. Kim, and A. Zeilinger, “Experimental realization of Dicke states of up to six qubits for multiparty quantum networking,” Phys. Rev. Lett. 103, 020503 (2009). 25. W. Wieczorek, C. Schmid, N. Kiesel, R. Pohlner, O. Gühne and H. Weinfurter, “Experimental observation of an entire family of four-photon entangled states,” Phys. Rev. Lett. 101, 010503 (2008). 26. C. Schmid, N. Kiesel, W. Laskowski, W. Wieczorek, M. Żukowski, and H. Weinfurter, “Discriminating multipartite entangled states,” Phys. Rev. Lett. 100, 200407 (2008). 27. C. K. Hong, Z. Y. Ou, and L. Mandel, “Measurement of subpicosecond time intervals between two photons by interference,” Phys. Rev. Lett. 59, 2044 (1987).


Introduction
Multi-particle entanglement states provide an important resource in quantum information and computing.Therefore, efficient preparation of these entangled states, e.g., Greenberger-Horne-Zeilinger(GHZ) states, cluster states and Dicke states, is an important task in experiment.The violations of local hidden variable theory for multipartite entangled states become the criteria of some Device-Independent (DI) quantum information processing tasks, such as the security of quantum key distribution (QKD) [1,2], decreasing the computation complexity [3,4] and the validity of random number generation [5], etc.
Observations of violations of local realism in the case of multipartite correlations are a challenging task because of the lack of handy Bell inequalities for multipartite systems, .
For two-qubit system, the Clauser-Horne-Shimony-Holt (CHSH) inequality [6] has a simple structure and is easy to observe the violation of local hidden variable theory experimentally.For arbitrary many observers, each choosing between two local dichotomic observables, the complete set of tight CHSH-type Bell inequalities has been obtained [7][8][9].Such inequalities have been pointed out to possess a common structure [10].However, the explicit expressions of Bell inequalities are too complicate to be used to verify the violation of local realism.The multipartite Mermin-Ardehali-Belinskii-klyshko (MABK) inequalities have the explicit expressions, however, the multipartite MABK inequality has 2 N terms [11][12][13] for N-partite system, it is not convenient to use MABK inequalities to check the nonlocality of a multipartite entangled states if the number of the particles is large.The multipartite Bell inequalities involving only two-body correlations still reveal the Bell-nonlocality in many-body system.Those Bell inequalitites open a way to verify multipartite Bell-nonlocality experimentally [14,15].
The less the number of terms of a Bell inequality is, the less difficulty of the implementation of nonlocality for multipartite entangled states is.Based on the geometrical properties of correlation polytopes [16], the structural features of CHSH-type Bell inequalities are found [17].Furthermore, the multipartite CHSH-type Bell inequalities with four terms are proposed.Therefore, it is possible to propose the experimental scheme to observe the violation of local realism for multipartite entangled states.
As a kind of important multipartite states which naturally arise in symmetric systems [18], #247024 Dicke states are highly persistent against photon loss and projective mesurements [19].These states possess high level multipartite entanglement.Recent researches also demonstrate that they are optimal for quantum metrology [20,21] and easy to quantify the entanglement depth for many-body systems [22].For these reasons, many works have been done on preparing the high quality Dicke states.In the optical system, the four-photon symmetric Dicke state with a fidelity of 0.844 ± 0.008 was prepared in experiment by N. Kiesel et al in 2007 [19], and the six-photon case was simultaneously realized by W. Wieczorek et al. [23] and R. Prevedel et al. [24].However, the general method used to detect the entanglement of Dicke states can not reveal the violation of local realism [19,20,[23][24][25].
In this work, we report an experimental demonstration of the local realism of the four-photon Dicke state D (2) 4 .Moreover, the Bell-type inequality we put forward has only four terms.It is more simple and easier to be realized in experiment than the one in [26].crystal is pumped by ultraviolet (UV) pulses to generate the four-photon scalar product state.Then they are equally distributed onto four spatial modes 'c', 'd', 'e' and 'f' by three beam splitters (BSs) behind interference filters (IF, △λ =3 nm, λ =780 nm).Polarization analysis (PA) in each basis is performed by using a quarter-wave plate (QWP) and a half-wave plate (HWP) in front of the polarizing beam splitter (PBS), and the photons are detected by the avalanche photo-diodes (APD).

Experiment
In our experiment, the frequency-doubled ultraviolet (UV) pulses (390 nm, 76 MHz repetition rate, 400 mW average power) from a mode-locked Ti:sapphire laser are used to pump a type-I beta-barium-borate (BBO) crystal (6 × 6 × 2 mm 3 ,θ = 29.9• ).This result in four horizontal polarization photons in a single pulse, After passing through the 45 • rotated half-wave plate1 (HWP1), the polarization of photons in mode 'a' is changed from horizonal orientation to vertical orientation.By adjusting a good Hong-Ou-Mandel-type interference [27] (the visibility of the interference is about 0.97), we removed the path information of photons in both modes (mode 'a' and mode 'b') and obtained four indistinguishable photons.As Fig. 1 shown, three Beam Splitters distribute them equally onto four spatial modes ('c', 'd', 'e', 'f').At last, only the four photon coincidence counts are recorded.Then we can get the two excitations four-photon Dicke state D By performing the standard tomography, we get the fidelity of state is 0.904 ± 0.004, which is better than the previous published results (details in Fig. 2).This is mainly due to the photon source we used.For our experiment setup, the photons are generated from the type-I nonlinear SPDC, then a HOM type interference with high visibility guarantees a good identity in their spatio-temporal mode structure.

Local realism
The Bell inequality we construct is devised by the method in [17].The inequality is given by where the local observables Âi , Bi , Ĉi and Di have the form: Xi = x i •σ , where By numerical computation, the maximal expectation value of Eq. ( 3) is given by 3.054 for Dicke state, while the coefficients of the local observables are given in Table 1: By adjusting the angles of the QWP and the HWP before the PBS, we can realize the measurement of the local observable, and the detections of the two outputs of PBS are corresponding to the projection measurement of its two eigenstates respectively.The 16 (four Table 1.The coefficients of the local observables.3), which are given by 0.6443 ± 0.0168, 0.4683 ± 0.0160, 0.6315 ± 0.0165 and −0.6588 ± 0.0167 (Fig. 3).When plugging them into the left of the inequality, we get a result of 2.403 ± 0.033.The threshold for the local realistic model of these correlations is less or equal to 2, and our experiment violates it by 12σ .Errors are mainly due to the time uncertainty of the photon pairs generated in BBO.The coincidence counts obey a Poisson distribution.

Conclusions
In summary, we have prepared a four-photon symmetric Dicke state with high fidelity by noncolinear SPDC process and high-visibility HOM interference.Then we demonstrate the nonlocal realism of the Dicke state.The confidence of violation is 12σ in our experiment.The new Belltype inequality we use only involves four correlation functions, i.e. we need the least measurements compared to other inequalities [26].And the term number will remain unchanged with the increasing of the size of system, so it is efficient for multi-photon experiment.

Fig. 1 .
Fig.1.Experimental setup for Dicke state preparation.A type-I beta-barium-borate (BBO) crystal is pumped by ultraviolet (UV) pulses to generate the four-photon scalar product state.Then they are equally distributed onto four spatial modes 'c', 'd', 'e' and 'f' by three beam splitters (BSs) behind interference filters (IF, △λ =3 nm, λ =780 nm).Polarization analysis (PA) in each basis is performed by using a quarter-wave plate (QWP) and a half-wave plate (HWP) in front of the polarizing beam splitter (PBS), and the photons are detected by the avalanche photo-diodes (APD).

6 (
|HHVV + |HV HV + |V HHV + |HVV H + |V HV H + |VV HH ), (2) the four entries in the state vector indicate the horizontal (H) or vertical (V) polarizations of the photons in one mode.For example, |HHVV = |H d ⊗ |H c ⊗ |V e ⊗ |V f denotes that the photons of mode 'c', mode 'd' are horizontal polarization and the photons mode 'e', mode 'f' are vertical polarization.For the purpose of obtaining high interference visibility, all the photons are coupled into single mode fibers in our experiment.Even though, nearly 23 four-fold coincidence counts can collect in one minute and this is enough to perform the full tomography.

Fig. 2 .
Fig. 2. State tomography.Histograms of the density matrix for the ideal state and the real part of the density matrix derived from the measurement data.
photon coincidence) measurements of D1 (D2), D3 (D4), D5 (D6) and D7 (D8) are combined together to obtain the values of the four terms in Eq.(3), which are given by 0.6443 ± 0.0168, 0.4683 ± 0.0160, 0.6315 ± 0.0165 and −0.6588 ± 0.0167 (Fig.3).When plugging them into the left of the inequality, we get a result of 2.403 ± 0.033.The threshold for the local realistic model of these correlations is less or equal to 2, and our experiment violates it by 12σ .Errors are mainly due to the time uncertainty of the photon pairs generated in BBO.The coincidence counts obey a Poisson distribution.