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Investigation of Coriolis Perturbations on the ro-vibrational ν1 Band of H2CO with fs-CARS

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Abstract

Experiment and simulation of fs-CARS signals from the ν1 band of formaldehyde including a model for ‘Coriolis’ interactions are presented. ‘Coriolis’ coupling coefficients and energy shifts are derived from the experiments by a least-square fit.

© 2006 Optical Society of America

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