Abstract.
We study two-photon double ionization of helium in its ground state at sufficiently low laser intensities so that three and more photon absorptions are negligible. In the regime where sequential ionization dominates, the two-photon double ionization one-electron energy spectrum exhibits a well defined double peak structure directly related to the electron-electron correlation in the ground state. We demonstrate that when helium is exposed to subfemtosecond or attosecond pulses, both peaks move and their displacement is a signature of the time needed by the He+ orbital to relax after the ejection of the first electron. This result rests on the numerical solution of the corresponding non-relativistic time-dependent Schrödinger equation.
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At 45 eV, the result obtained with the B-spline basis differs from a previous one given by S. Laulan, H. Bachau, in the Proceedings of the International conference on “Electron and photon impact ionisation and related topics” (Metz, 2002) which will be published by The Institute of Physics (IOP) series 171. This previous result has been obtained by using the interaction picture
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Received: 17 January 2003, Published online: 18 March 2003
PACS:
32.80.Rm Multiphoton ionization and excitation to highly excited states (e.g., Rydberg states) - 32.80.Dz Autoionization
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Piraux, B., Bauer, J., Laulan, S. et al. Probing electron-electron correlation with attosecond pulses. Eur. Phys. J. D 26, 7–13 (2003). https://doi.org/10.1140/epjd/e2003-00063-3
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DOI: https://doi.org/10.1140/epjd/e2003-00063-3