Abstract.
The kinetics of aggregate growth through reversible migrations between any two aggregates is studied. We propose a simple model with the symmetrical migration rate kernel \(K(k;j)\propto (kj)^\upsilon\) at which the monomers migrate from the aggregates of size k to those of size j. The results show that for the \(\upsilon \leq 3/2\) case, the aggregate size distribution approaches a conventional scaling form; moreover, the typical aggregate size grows as \(t^{1 / (3 - 2\upsilon )}\) in the \( \upsilon < 3/2\) case and as \(\exp(C_1 t)\) in the \(\upsilon = 3/2\) case. We also investigate another simple model with the asymmetrical rate kernel \(K(k;j)\propto k^\mu j^\nu\) (\(\mu \neq \nu\)), which exhibits some scaling properties quite different from the symmetrical one. The aggregate size distribution satisfies the conventional scaling form only in the case of \(\mu < \nu\) and \(\mu + \nu < 2\), and the typical aggregate size grows as \(t^{2-\mu-\nu}\).
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Received: 14 October 2003, Published online: 23 December 2003
PACS:
82.20.-w Chemical kinetics and dynamics - 68.43.Jk Diffusion of adsorbates, kinetics of coarsening and aggregation - 89.75.Da Systems obeying scaling laws
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Ke, J., Lin, Z. & Zhuang, Y. Aggregate size distributions in migration driven growth models. Eur. Phys. J. B 36, 423–428 (2003). https://doi.org/10.1140/epjb/e2003-00362-5
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DOI: https://doi.org/10.1140/epjb/e2003-00362-5