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Seven Modern Trends in the DeNOx Catalyst Development

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Abstract

As a result of anthropogenic activities, millions of tons of nitrogen oxides (NOx = NO, NO2) are emitted into the atmosphere every year, which poses a serious threat to human health. The catalytic neutralization of vehicle exhaust gases and industrial waste gases is the most effective solution to the problem of man-made NOx emissions. To date, there are a number of catalytic technologies for the removal of nitrogen oxides; however, their use is limited because of their low efficiency at temperatures of 100–300°C. This review is devoted to current trends in the development of highly active catalysts for the removal of nitrogen oxides from vehicle exhaust gases and waste gases of the chemical industry at temperatures below 300°C. The main attention is paid to new catalytic systems based on mixed oxides, hydrotalcites, perovskites, small-pore zeolites, metal–organic frameworks (MOF), and natural minerals and clays, as well as to hybrid catalysts.

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ACKNOWLEDGMENTS

Scientific Schools Development Program by Zelinsky Institute of Organic Chemistry is gratefully acknowledged.

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Authors and Affiliations

  1. N.D. Zelinsky Institute of Organic Chemistry, Russian Academy of Sciences, 119991, Moscow, Russia

    A. I. Mytareva, D. A. Bokarev & A. Yu. Stakheev

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  1. A. I. Mytareva
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  2. D. A. Bokarev
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  3. A. Yu. Stakheev
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Correspondence to A. I. Mytareva.

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Translated by O. Kadkin

Abbreviations and notation: SCR, selective catalytic reduction; LDH, layered double hydroxide; LDO, layered double oxide; HTT, hydrothermal treatment; IO, ion exchange; SSIO, solid-state ion exchange; HP, homogeneous precipitation; ATP, attapulgite; MMT, montmorillonite; DPC, dolomite–palygorskite clay; OC, organic clay; MOF, metal–organic framework; PILC, pillared interlayered clay.

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Mytareva, A.I., Bokarev, D.A. & Stakheev, A.Y. Seven Modern Trends in the DeNOx Catalyst Development. Kinet Catal 62, 1–32 (2021). https://doi.org/10.1134/S0023158420060105

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  • DOI: https://doi.org/10.1134/S0023158420060105

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