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Analysis of the Effect of Restrictions on Isotopes 232,234,236U in Marketable LEU on the Choice of Methods for Enriching Reprocessed Uranium in Cascades of Centrifuges

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Abstract

The study addresses the problems of reprocessed uranium re-enrichment. It is shown that, in the most general formulation, the problem of reprocessed uranium re-enrichment that meets all the requirements on the content of even isotopes and the conditions of spending a given amount of initial reprocessed uranium for production of unit mass of the product cannot be solved in a three-flow cascade of centrifuges or in the simplest versions of double cascades. The possibility of solving the formulated problem in a modified double cascade scheme with a low-enriched uranium (LEU) diluter is demonstrated. The results of numerical experiments showed that it is possible to obtain marketable LEU in the studied version of the double cascade after spending a given amount of reprocessed uranium and meeting different constraints on 232U concentration in the product, including even stricter constraints than those currently accepted at separation plants.

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REFERENCES

  1. E. A. Andrianova, V. D. Davidenko, and V. F. Tsibul’skii, At. Energy 118, 301 (2015).

  2. A. A. Orlov, A. V. Kravchenko, E. S. Titov, and A. Ya. Lebedev, Izv. Vyssh. Uchebn. Zaved., Fiz. 58 (2), 35 (2015).

    Google Scholar 

  3. A. M. Pavlovichev, V. I. Pavlov, Yu. M. Semchenkov, E. G. Kudryavtsev, Yu. S. Fedorov, and B. A. Bibichev, At. Energy 101, 863 (2006).

    Article  Google Scholar 

  4. V. Yu. Blandinskii, A. V. Grol’, A. A. Dudnikov, V. A. Nevinitsa, P. A. Fomichenko, A. Yu. Smirnov, and G. A. Sulaberidze, Vopr. At. Nauki Tekh., Ser. Yad.-Reakt. Konst., No. 1, 65 (2018).

  5. A. Yu. Smirnov, G. A. Sulaberidze, P. N. Alekseev, A. A. Dudnikov, V. A. Nevinitsa, V. N. Proselkov, and A. V. Chibinyaev, Vopr. At. Nauki Tekh., Ser.: Fiz. Yad. Reakt., No. 4, 70 (2010).

  6. K. Hida, S. Kusuno, and T. Seino, Nucl. Technol. 75, 148 (1986).

    Article  Google Scholar 

  7. J. R. Coleman and T. W. Knight, Nucl. Eng. Design 240, 1028 (2010).

    Article  Google Scholar 

  8. A. I. Kislov, A. A. Titov, A. M. Dmitriev, A. E. Sintsov, and A. V. Romanov, Yad. Rad. Bezopasn., Spec. Iss. (2012).

    Google Scholar 

  9. V. N. Prusakov, A. A. Sazykin, L. Yu. Sosnin, D. V. Utrobin, and A. N. Chel’tsov, At. Energy 105, 194 (2008).

    Article  Google Scholar 

  10. A. Yu. Smirnov, G. A. Sulaberidze, V. A. Nevinitsa, et al., Yad. Fiz. Inzhin. 3, 396 (2012).

    Google Scholar 

  11. V. A. Palkin, At. Energy 115, 32 (2013).

  12. G. A. Sulaberidze, V. D. Borisevich, and Q. X. Xie, Theor. Found. Chem. Eng. 40, 5 (2006).

    Article  Google Scholar 

  13. V. A. Palkin, Persp. Mater., No. 8, 11 (2010).

  14. A. Yu. Smirnov and G. A. Sulaberidze, At. Energy 117, 44 (2014).

    Article  Google Scholar 

  15. V. A. Palkin, At. Energy 118, 191 (2015).

  16. V. A. Palkin, At. Energy 121, 197 (2016).

  17. V. A. Palkin and E. V. Maslyukov, Theor. Found. Chem. Eng. 50, 711 (2016).

    Article  Google Scholar 

  18. V. A. Palkin, At. Energy 121, 43 (2016).

  19. A. Yu. Smirnov, V. E. Gusev, G. A. Sulaberidze, V. A. Nevinitsa, and P. A. Fomichenko, Vestn. MIFI 7, 449 (2018).

    Google Scholar 

  20. G. A. Sulaberidze, V. A. Palkin, V. D. Borisevich, et al., Cascade Theory for the Separation of Binary and Multicomponent Isotopic Mixtures, The School-Book, Ed. by V. D. Borman (NIYaU MIFI, Moscow, 2011) [in Russian].

  21. A. A. Orlov, A. F. Tsimbalyuk, and R. V. Malyugin, Sep. Purif. Rev. 46, 81 (2016).

    Article  Google Scholar 

  22. A. A. Orlov and R. V. Malyugin, Adv. Mater. Res. 1084, 338 (2015).

    Article  Google Scholar 

  23. A. A. Orlov, A. F. Tsimbalyuk, and R. V. Malyugin, Vestn. MIFI 5, 558 (2016).

    Google Scholar 

  24. A. A. Orlov and R. V. Malyugin, Sovrem. Naukoemk. Tekhnol., Region. Prilozh., No. 3, 89 (2014).

  25. V. A. Palkin, A. Yu. Smirnov, and G. A. Sulaberidze, in Proceedings of the SPLG-2010 Conference, St. Petersburg, Russia, June 13–18, 2010, p. 142.

  26. G. A. Sulaberidze, V. D. Borisevich, and Ts.-S. Se, in Proceedings of the 9th All-Russia Conference on Physico-Chemical Processes during Atom and Molecule Selection, Zvenigorod, Russia, Oct. 4–8, 2004 (TsNIIatominform, TRINITI, Troitsk, Moscow, 2004).

  27. V. A. Zhurin, V. V. Vodolazskikh, V. I. Shchelkanov, V. A. Palkin, and N. P. Glukhov, RF Patent No. 2399971 (2009).

  28. V. V. Vodolazskikh, V. A. Kozlov, V. I. Mazin, M. I. Sterkhov, and V. V. Shidlovskii, RF Patent No. 2282904 (2006).

  29. A. A. Sazykin, in Proceedings of the 5th All-Russia Conference on Physico-Chemical Processes during Atom and Molecule Selection, Zvenigorod, Russia (TsNIIatominform, Moscow, 2000), p. 51.

  30. A. A. Dudnikov, V. A. Nevinitsa, V. N. Proselkov, A. S. Sumarokova, P. A. Fomichenko, A. Yu. Smirnov, and G. A. Sulaberidze, At. Energy 119, 291 (2016).

    Article  Google Scholar 

  31. V. A. Nevinitsa, N. N. Ponomarev-Stepnoi, A. Yu. Smirnov, G. A. Sulaberidze, et al., Phys. At. Nucl. 73, 2264 (2010).

    Article  Google Scholar 

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Funding

This work was supported by the National Research Center Kurchatov Institute (Order on Performing Scientific Research Work no. 1879 of August 2, 2019).

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Correspondence to A. Yu. Smirnov.

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Translated by E. Baldina

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Smirnov, A.Y., Gusev, V.E., Sulaberidze, G.A. et al. Analysis of the Effect of Restrictions on Isotopes 232,234,236U in Marketable LEU on the Choice of Methods for Enriching Reprocessed Uranium in Cascades of Centrifuges. Phys. Atom. Nuclei 84, 1500–1507 (2021). https://doi.org/10.1134/S1063778821080184

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  • DOI: https://doi.org/10.1134/S1063778821080184

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