Magnetic skyrmions, vortex-like topological spin textures, have attracted much attention in terms of both fundamental physics and spintronics applications. Thus far, skyrmions have been observed in thin-film multilayers with interfacial Dzyaloshinskii-Moriya interaction (DMI) and structurally-chiral magnets with bulk DMI. Recently, bulk-DMI-induced skyrmions have been observed above room temperature in Co-Zn-Mn alloys with a β-Mn-type chiral structure [1]. In most chiral magnets, however, skyrmions exist as a thermodynamically equilibrium state only in a narrow temperature and magnetic field region just below the magnetic transition temperature Tc. The limited region of the stable skyrmions is unfavorable for applications.
Here, we focused on β-Mn-type Co9Zn9Mn2 (Tc ~ 400 K) and performed small-angle neutron scattering, magnetic susceptibility and Lorentz transmission electron microscope measurements. We demonstrated that skyrmions persist over almost the whole temperature region below 400 K as a long-lived metastable state by performing a conventional field-cooling process. Once created, metastable skyrmions survive above room temperature after removal of magnetic field [2]. These findings exemplify the topological robustness of the once-created skyrmions and provide a significant step toward applications of skyrmions in bulk chiral magnets.
In the presentation, we will discuss the details of the above observations, and also show novel skyrmion states in Co-Zn-Mn alloys with other chemical compositions.
[1] Y. Tokunaga et al., Nat. Commun. 6, 7638 (2015).
[2] K. Karube et al., Phys. Rev. Mater. 1, 074405 (2017).
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