Spinon Heat Transport in the Three-Dimensional Quantum Magnet PbCuTe2O6

Xiaochen Hong, Matthias Gillig, Abanoub R. N. Hanna, Shravani Chillal, A. T. M. Nazmul Islam, Bella Lake, Bernd Büchner, and Christian Hess
Phys. Rev. Lett. 131, 256701 – Published 18 December 2023

Abstract

Quantum spin liquids (QSLs) are novel phases of matter which remain quantum disordered even at the lowest temperature. They are characterized by emergent gauge fields and fractionalized quasiparticles. Here we show that the sub-kelvin thermal transport of the three-dimensional S=1/2 hyperhyperkagome quantum magnet PbCuTe2O6 is governed by a sizeable charge-neutral fermionic contribution which is compatible with the itinerant fractionalized excitations of a spinon Fermi surface. We demonstrate that this hallmark feature of the QSL state is remarkably robust against sample crystallinity, large magnetic field, and field-induced magnetic order, ruling out the imitation of QSL features by extrinsic effects. Our findings thus reveal the characteristic low-energy features of PbCuTe2O6 which qualify this compound as a true QSL material.

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  • Received 19 July 2023
  • Accepted 15 November 2023

DOI:https://doi.org/10.1103/PhysRevLett.131.256701

© 2023 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Xiaochen Hong1,2, Matthias Gillig2, Abanoub R. N. Hanna3,4, Shravani Chillal4, A. T. M. Nazmul Islam4, Bella Lake3,4, Bernd Büchner2,5, and Christian Hess1,2,*

  • 1Fakultät für Mathematik und Naturwissenschaften, Bergische Universität Wuppertal, Gaußstraße 20, 42119 Wuppertal, Germany
  • 2Leibniz-Institute for Solid State and Materials Research (IFW-Dresden), Helmholtzstraße 20, 01069 Dresden, Germany
  • 3Institut für Festkörperforschung, Technische Universität Berlin, Hardenbergstraße 36, 10623 Berlin, Germany
  • 4Helmholtz-Zentrum Berlin für Materialien und Energie, Hahn-Meitner Platz 1, 14109 Berlin, Germany
  • 5Institute of Solid State and Materials Physics and Würzburg-Dresden Cluster of Excellence ct.qmat, Technische Universität Dresden, 01062 Dresden, Germany

  • *c.hess@uni-wuppertal.de

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Issue

Vol. 131, Iss. 25 — 22 December 2023

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