Mode-coupling theory for tagged-particle motion of active Brownian particles

Julian Reichert, Suvendu Mandal, and Thomas Voigtmann
Phys. Rev. E 104, 044608 – Published 19 October 2021

Abstract

We derive a mode-coupling theory (MCT) to describe the dynamics of a tracer particle that is embedded in a dense system of active Brownian particles (ABPs) in two spatial dimensions. The ABP undergo translational and rotational Brownian motion and are equipped with a fixed self-propulsion speed along their orientational vector that describes their active motility. The resulting equations of motion for the tagged-particle density-correlation functions describe the various cases of tracer dynamics close to the glass transition: that of a single active particle in a glass-forming passive host suspensions, that of a passive colloidal particle in a suspension of ABP, and that of active tracers in a bath of active particles. Numerical results are presented for these cases assuming hard-sphere interactions among the particles. The qualitative and quantitative accuracy of the theory is tested against event-driven Brownian dynamics (ED-BD) simulations of active and passive hard disks. Simulation and theory are found in quantitative agreement, provided one adjusts the overall density (as known from the passive description of glassy dynamics), and allows for a rescaling of self-propulsion velocities in the active host system. These adjustments account for the fact that ABP-MCT generally overestimates the tendency for kinetic arrest. We confirm in the simulations a peculiar feature of the transient and stationary dynamical density-correlation functions regarding their lack of symmetry under time reversal, demonstrating the nonequilibrium nature of the system and how it manifests itself in the theory.

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  • Received 2 August 2021
  • Accepted 5 October 2021

DOI:https://doi.org/10.1103/PhysRevE.104.044608

©2021 American Physical Society

Physics Subject Headings (PhySH)

Polymers & Soft MatterStatistical Physics & ThermodynamicsPhysics of Living Systems

Authors & Affiliations

Julian Reichert1, Suvendu Mandal2,*, and Thomas Voigtmann1,2

  • 1Institut für Materialphysik im Weltraum, Deutsches Zentrum für Luft- und Raumfahrt (DLR), 51170 Köln, Germany
  • 2Department of Physics, Heinrich-Heine Universität Düsseldorf, Universitätsstrasse 1, 40225 Düsseldorf, Germany

  • *Current address: Institut für Physik der kondensierten Materie, Technische Universität Darmstadt, 64289 Darmstadt, Germany.

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Issue

Vol. 104, Iss. 4 — October 2021

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