Electronic wave functions and optical transitions in (In,Ga)As/GaP quantum dots

C. Robert, K. Pereira Da Silva, M. O. Nestoklon, M. I. Alonso, P. Turban, J.-M. Jancu, J. Even, H. Carrère, A. Balocchi, P. M. Koenraad, X. Marie, O. Durand, A. R. Goñi, and C. Cornet
Phys. Rev. B 94, 075445 – Published 30 August 2016

Abstract

We study the complex electronic band structure of low In content InGaAs/GaP quantum dots. A supercell extended-basis tight-binding model is used to simulate the electronic and the optical properties of a pure GaAs/GaP quantum dot modeled at the atomic level. Transitions between hole states confined into the dots and several XZ-like electronic states confined by the strain field in the GaP barrier are found to play the main role on the optical properties. Especially, the calculated radiative lifetime for such indirect transitions is in good agreement with the photoluminescence decay time measured in time-resolved photoluminescence in the µs range. Photoluminescence experiments under hydrostatic pressure are also presented. The redshift of the photoluminescence spectrum with pressure is also in good agreement with the nature of the electronic confined states simulated with the tight-binding model.

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  • Received 9 March 2016
  • Revised 19 July 2016

DOI:https://doi.org/10.1103/PhysRevB.94.075445

©2016 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

C. Robert1,2, K. Pereira Da Silva3,4, M. O. Nestoklon5, M. I. Alonso3, P. Turban6, J.-M. Jancu1, J. Even1, H. Carrère2, A. Balocchi2, P. M. Koenraad7, X. Marie2, O. Durand1, A. R. Goñi3,8, and C. Cornet1

  • 1Université Européenne de Bretagne, INSA, FOTON UMR 6082, 35708 Rennes, France
  • 2Université de Toulouse, INSA-CNRS-Université Paul Sabatier (UPS), Laboratoire de physique et chimie de nano-objets (LPCNO), 135 Avenue Rangueil, 31077 Toulouse, France
  • 3Institut de Ciència de Materials de Barcelona, Consejo Superior de Investigaciones Científicas (ICMAB-CSIC), Campus Universitat Autònoma de Bellaterra (UAB), 08193 Bellaterra, Spain
  • 4Departamento de Física, Universidade Federal do Ceará, P.O. Box 6030, Fortaleza–CE, 60455–970, Brazil
  • 5Ioffe Institute, St. Petersburg 194021, Russia
  • 6Institut de physique de Rennes (IPR), UMR 6251, CNRS-Université de Rennes I, Campus de Beaulieu 35042 Rennes Cedex, France
  • 7Department of Applied Physics, Eindhoven University of Technology, P.O. Box 513, 5600 MB Eindhoven, The Netherlands
  • 8Institució Catalana de Recerca i Estudis Avançats (ICREA), Passeig Lluís Companys 23, 08010 Barcelona, Spain

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Issue

Vol. 94, Iss. 7 — 15 August 2016

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