Abstract
SrYbO is a geometrically frustrated rare-earth magnet, which presents a variety of interrelated magnetic phenomena. The magnetic Yb ions () form potentially frustrated “zigzag” chains along the axis, arranged in a honeycomb fashion in the plane. Heat capacity reveals a magnetic phase transition at K. The magnetic structure was solved by polarized neutron diffraction and found to be noncollinear with a reduction of the ordered spin moment from the full ionic moment. The low-energy excitations, which were measured by inelastic neutron scattering reveal diffuse scattering both above and below . Heat capacity and magnetocaloric effect were performed to map out the magnetic phase diagram as a function of magnetic field and temperature and show a complicated series of states. Altogether, the results suggest that the magnetic interactions in SrYbO compete with each other and with the single-ion anisotropy to produce a highly degenerate ground state manifold that suppresses the magnetic order, broadens the excitations and gives rise to a complex phase diagram.
1 More- Received 29 May 2012
DOI:https://doi.org/10.1103/PhysRevB.86.064203
©2012 American Physical Society