Structural and dynamical study of moment localization in β-Mn1xInx

J. R. Stewart, A. D. Hillier, J. M. Hillier, and R. Cywinski
Phys. Rev. B 82, 144439 – Published 27 October 2010

Abstract

We have used neutron-scattering and muon spin relaxation (μSR) to investigate the structural and magnetic properties of the β phase of elemental manganese doped with dilute amounts of indium. β-Mn is an example of a topologically frustrated antiferromagnetically correlated metal—but which remains paramagnetic at all temperatures. The addition of In to β-Mn results in a vast volume expansion of the lattice and would therefore be expected to have a major effect on the stability and localization of the Mn moment as observed in, for example, Ru- and Al-doped β-Mn alloys. We find that In doping in β-Mn results in a short-range ordered spin-glasslike ground state, similar to that of Al-doped β-Mn but with residual low-frequency spin fluctuations. This is in contrast to Ru doping which results in the stabilization of a long-range-ordered Mn moment

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  • Received 30 July 2010

DOI:https://doi.org/10.1103/PhysRevB.82.144439

©2010 American Physical Society

Authors & Affiliations

J. R. Stewart* and A. D. Hillier

  • ISIS, STFC, Rutherford Appleton Laboratory, Didcot OX11 0QX, United Kingdom

J. M. Hillier

  • Department of Education, Oxford University, 15 Norham Gardens, Oxford OX2 6PY, United Kingdom

R. Cywinski

  • School of Applied Sciences, University of Huddersfield, Queensgate, Huddersfield HD1 3DH, United Kingdom

  • *ross.stewart@stfc.ac.uk
  • Institut Laue-Langevin, 6, rue Jules Horowitz, F-38042 Grenoble, France.

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Issue

Vol. 82, Iss. 14 — 1 October 2010

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