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Polariton-assisted long-distance energy transfer between excitons in two-dimensional semiconductors

Tuomas Pajunpää, Fedor Nigmatulin, Suvi-Tuuli Akkanen, Henry Fernandez, Gerrit Groenhof, and Zhipei Sun
Phys. Rev. B 109, 195409 – Published 3 May 2024

Abstract

Strong exciton-photon coupling offers an effective path for polariton-mediated long-distance coherent energy transfer (ET) between excitonic states. Here, we demonstrate strong coupling between excitons in WS2 monolayers, MoS2 bilayer, and photons in a tunable optical microcavity at room temperature. Full quantum dynamics simulations based on experimental parameters show that the demonstrated system provides an efficient and adjustable platform for ultrafast polariton-assisted ET between the excitons in two-dimensional materials when the separation between them exceeds 1µm.

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  • Received 5 January 2024
  • Revised 9 April 2024
  • Accepted 11 April 2024

DOI:https://doi.org/10.1103/PhysRevB.109.195409

©2024 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied PhysicsAtomic, Molecular & Optical

Authors & Affiliations

Tuomas Pajunpää1, Fedor Nigmatulin1, Suvi-Tuuli Akkanen1, Henry Fernandez1,*, Gerrit Groenhof2, and Zhipei Sun1,†

  • 1QTF Centre of Excellence, Department of Electronics and Nanoengineering, Aalto University, FI-00076 Aalto, Finland
  • 2Nanoscience Center, Department of Chemistry, P.O. Box 35, FI-40014 University of Jyväskylä, Finland

  • *henryfernandez09@live.com
  • zhipei.sun@aalto.fi

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Issue

Vol. 109, Iss. 19 — 15 May 2024

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