Breakdown of linear spin-wave theory and existence of spinon bound states in the frustrated kagome-lattice antiferromagnet

K. Matan, T. Ono, S. Ohira-Kawamura, K. Nakajima, Y. Nambu, and T. J. Sato
Phys. Rev. B 105, 134403 – Published 6 April 2022

Abstract

The spin dynamics of the spin-1/2 kagome-lattice antiferromagnet Cs2Cu3SnF12 is studied using high-resolution, time-of-flight inelastic neutron scattering. The flat mode, a characteristic of the frustrated kagome antiferromagnet, and the low-energy dispersive mode, which is dominated by magnons, can be well described by the linear spin-wave theory. However, the theory fails to describe three weakly dispersive modes between 9 and 14 meV. These modes could be attributed to two-spinon bound states, which decay into free spinons away from the zone center and at a high temperature, giving rise to continuum scattering.

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  • Received 2 February 2022
  • Revised 3 March 2022
  • Accepted 18 March 2022

DOI:https://doi.org/10.1103/PhysRevB.105.134403

©2022 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

K. Matan1,2,*, T. Ono3, S. Ohira-Kawamura4, K. Nakajima4, Y. Nambu5,6,7, and T. J. Sato8

  • 1Department of Physics, Faculty of Science, Mahidol University, Bangkok 10400, Thailand
  • 2ThEP, Commission of Higher Education, Bangkok 10400, Thailand
  • 3Department of Physical Science, School of Science, Osaka Prefecture University, Sakai, Osaka 599-8531, Japan
  • 4Materials and Life Science Division, J-PARC Center, Tokai, Ibaraki 319-1195, Japan
  • 5Institute for Materials Research, Tohoku University, Sendai 980-8577, Japan
  • 6FOREST, Japan Science and Technology Agency, Kawaguchi, Saitama 332-0012, Japan
  • 7Organization for Advanced Studies, Tohoku University, Sendai 980-8577, Japan
  • 8Institute of Multidisciplinary Research for Advanced Materials, Tohoku University, 2-1-1 Katahira, Sendai, Miyagi 980-8577, Japan

  • *kittiwit.mat@mahidol.ac.th

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Issue

Vol. 105, Iss. 13 — 1 April 2022

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