${\mathrm{Cu}}_2{\mathrm{OSeO}}_3$ is an insulating skyrmion-host material with a magnetoelectric coupling giving rise to an electric polarization with a characteristic dependence on the magnetic-field $\vec{H}$. We report a magnetic force microscopy imaging of the helical real-space spin structure on the surface of a bulk single crystal of ${\mathrm{Cu}}_2{\mathrm{OSeO}}_3$. In the presence of a magnetic field, the helimagnetic order, in general, reorients and acquires a homogeneous component of the magnetization, resulting in a conical arrangement at larger fields. We investigate this reorientation process at a temperature of 10 K for fields close to the crystallographic $\langle 110\rangle$ direction that involves a phase transition at $H_{c1}$. Experimental evidence is presented for the formation of magnetic domains in real space as well as for the microscopic origin of relaxation events that accompany the reorientation process. In addition, the electric polarization is measured by means of Kelvin-probe force microscopy. We show that the characteristic field dependency of the electric polarization originates in this helimagnetic reorientation process. Our experimental results are well described by an effective Landau theory previously invoked for MnSi, that captures the competition between magnetocrystalline anisotropies and Zeeman energy.

• Received 6 May 2020
• Accepted 30 June 2020

DOI:https://doi.org/10.1103/PhysRevB.102.024426