Absolute Ionization Rates of Multielectron Transition Metal Atoms in Strong Infrared Laser Fields

Marc Smits, C. A. de Lange, Albert Stolow, and D. M. Rayner
Phys. Rev. Lett. 93, 213003 – Published 15 November 2004

Abstract

We report on nonresonant strong field ionization of the multielectron transition metal atoms V, Nb, Ta, Ni, and Pd. Operating in the adiabatic regime (λ=1.5μm), we quantitatively determined both (i) the first charge state saturation intensities and (ii) the absolute ionization rates for intensities ranging from threshold up to 3×1014W/cm2. We observed a dramatic suppression of ionization relative to single active electron approximation expectations. We suggest that this derives from dynamic polarization or screening effects within the multielectron atom, stressing a need for many-body theories of strong field ionization.

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  • Received 31 May 2004

DOI:https://doi.org/10.1103/PhysRevLett.93.213003

©2004 American Physical Society

Authors & Affiliations

Marc Smits1, C. A. de Lange1, Albert Stolow2,*, and D. M. Rayner2,†

  • 1Department of Physics and Astronomy, Vrije Universiteit Amsterdam, Netherlands
  • 2Steacie Institute for Molecular Sciences, National Research Council Canada, 100 Sussex Drive, Ottawa, Ontario K1A 0R6 Canada

  • *Electronic address: albert.stolow@nrc-cnrc.gc.ca
  • Electronic address: david.rayner@nrc-cnrc.gc.ca

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Issue

Vol. 93, Iss. 21 — 19 November 2004

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