Unusual Magnetic State in Lithium-Doped MoS2 Nanotubes

D. Mihailovic, Z. Jaglicic, D. Arcon, A. Mrzel, A. Zorko, M. Remskar, V. V. Kabanov, R. Dominko, M. Gaberscek, C. J. Gómez-García, J. M. Martínez-Agudo, and E. Coronado
Phys. Rev. Lett. 90, 146401 – Published 9 April 2003

Abstract

We report on the very peculiar magnetic properties of an ensemble of very weakly coupled lithium-doped MoS2 nanotubes. The magnetic susceptibility χ of the system is nearly 3 orders of magnitude greater than in typical Pauli metals, yet there is no evidence for any instability which would alleviate this highly frustrated state. Instead, the material exhibits peculiar paramagnetic stability down to very low temperatures, with no evidence of a quantum critical point as T0 in spite of clear evidence for strongly correlated electron behavior. The exceptionally weak intertube interactions appear to lead to a realization of a near-ideal one-dimensional state in which fluctuations prevent the system from reordering magnetically or structurally.

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  • Received 2 January 2003

DOI:https://doi.org/10.1103/PhysRevLett.90.146401

©2003 American Physical Society

Authors & Affiliations

D. Mihailovic1, Z. Jaglicic2, D. Arcon1, A. Mrzel1, A. Zorko1, M. Remskar1, V. V. Kabanov1, R. Dominko3, M. Gaberscek3, C. J. Gómez-García4, J. M. Martínez-Agudo4, and E. Coronado4

  • 1Jozef Stefan Institute, Jamova 39, 1000 Ljubljana, Slovenia
  • 2Institute of Mathematics, Phyisics and Mechanics, Jadranska 19, 1000 Ljubljana, Slovenia
  • 3National Chemistry Institute, Hajdrihova 19, 1000 Ljubljana, Slovenia
  • 4Instituto de Ciencia Molecular, Departamento Quemica Inorganica, Universidad de Valencia, 46100 Burjasot, Spain

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Vol. 90, Iss. 14 — 11 April 2003

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