Correlated Motion of Electrons on the Au(111) Surface: Anomalous Acoustic Surface-Plasmon Dispersion and Single-Particle Excitations

L. Vattuone, M. Smerieri, T. Langer, C. Tegenkamp, H. Pfnür, V. M. Silkin, E. V. Chulkov, P. M. Echenique, and M. Rocca
Phys. Rev. Lett. 110, 127405 – Published 22 March 2013
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Abstract

The linear dispersion of the low-dimensional acoustic surface plasmon (ASP) opens perspectives in energy conversion, transport, and confinement far below optical frequencies. Although the ASP exists in a wide class of materials, ranging from metal surfaces and ultrathin films to graphene and topological insulators, its properties are still largely unexplored. Taking Au(111) as a model system, our combined experimental and theoretical study revealed an intriguing interplay between collective and single particle excitations, causing the ASP associated with the Shockley surface state to be embedded within the intraband transitions without losing its sharp character and linear dispersion.

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  • Received 8 October 2012

DOI:https://doi.org/10.1103/PhysRevLett.110.127405

© 2013 American Physical Society

Authors & Affiliations

L. Vattuone1, M. Smerieri1, T. Langer2, C. Tegenkamp2, H. Pfnür2, V. M. Silkin3,4,5, E. V. Chulkov3,4,6, P. M. Echenique3,4,6, and M. Rocca1

  • 1Dipartimento di Fisica dell’Universitá di Genova and IMEM-CNR Unitá Operativa di Genova, Via Dodecaneso 33, 15146 Genova, Italy
  • 2Institut für Festkörperphysik, Abteilung Atomare und Molekulare Strukturen, Leibniz Universität Hannover, Appelstraße 2, D-30167 Hannover, Germany
  • 3Departamento de Física de Materiales, Facultad de Ciencias Químicas, Universidad del País Vasco, Apartado 1072, 20080 San Sebastián/Donostia, Spain
  • 4Donostia International Physics Center (DIPC), Paseo de Manuel Lardizabal 4, 20018 San Sebastián/Donostia, Spain
  • 5IKERBASQUE, Basque Foundation for Science, 48011 Bilbao, Spain
  • 6Centro de Física de Materiales CFM-Materials Physics Center MPC, Centro Mixto CSIC-UPV/EHU, Paseo de Manuel Lardizabal 5, 20018 San Sebastián/Donostia, Spain

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Vol. 110, Iss. 12 — 22 March 2013

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