Nonconventional Spin Glass Transition in a Chemically Ordered Pyrochlore

D. K. Singh and Y. S. Lee
Phys. Rev. Lett. 109, 247201 – Published 10 December 2012
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Abstract

We report on the study of unusual spin glass properties in the geometrically frustrated pyrochlore Tb2Mo2O7, Tg24K. The analysis of the nonlinear part of dc and complex susceptibilities, near the glass transition regime, suggests the existence of a statistical distribution of relaxation times in short-range ordered ferromagnetic clusters. In addition, the magnetic spins are not sufficiently frozen below the glass transition temperature, which is apparently responsible for the nonequilibrium scaling behavior of the static critical exponents of nonlinear susceptibilities. Our report is expected to shed new light in understanding the freezing properties of frustrated pyrochlores with short-range ferromagnetic interactions.

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  • Received 23 July 2012

DOI:https://doi.org/10.1103/PhysRevLett.109.247201

© 2012 American Physical Society

Authors & Affiliations

D. K. Singh1,2,3,* and Y. S. Lee1

  • 1Department of Physics, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139, USA
  • 2NIST Center for Neutron Research, Gaithersburg, Maryland 20874, USA
  • 3Department of Materials Science and Engineering, University of Maryland, College Park, Maryland 20742, USA

  • *To whom all correspondence should be addressed. dsingh@nist.gov

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Issue

Vol. 109, Iss. 24 — 14 December 2012

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