Quantum Magnets under Pressure: Controlling Elementary Excitations in TlCuCl3

Ch. Rüegg, B. Normand, M. Matsumoto, A. Furrer, D. F. McMorrow, K. W. Krämer, H. -U. Güdel, S. N. Gvasaliya, H. Mutka, and M. Boehm
Phys. Rev. Lett. 100, 205701 – Published 21 May 2008

Abstract

We follow the evolution of the elementary excitations of the quantum antiferromagnet TlCuCl3 through the pressure-induced quantum critical point, which separates a dimer-based quantum disordered phase from a phase of long-ranged magnetic order. We demonstrate by neutron spectroscopy the continuous emergence in the weakly ordered state of a low-lying but massive excitation corresponding to longitudinal fluctuations of the magnetic moment. This mode is not present in a classical description of ordered magnets, but is a direct consequence of the quantum critical point.

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  • Received 20 March 2008

DOI:https://doi.org/10.1103/PhysRevLett.100.205701

©2008 American Physical Society

Authors & Affiliations

Ch. Rüegg1, B. Normand2,3, M. Matsumoto4, A. Furrer5, D. F. McMorrow1, K. W. Krämer6, H. -U. Güdel6, S. N. Gvasaliya5, H. Mutka7, and M. Boehm7

  • 1London Centre for Nanotechnology, University College London, London WC1E 6BT, United Kingdom
  • 2Département de Physique, Université de Fribourg, CH-1700 Fribourg, Switzerland
  • 3Theoretische Physik, ETH-Hönggerberg, CH-8093 Zürich, Switzerland
  • 4Department of Physics, Faculty of Science, Shizuoka University, Shizuoka 422-8529, Japan
  • 5Laboratory for Neutron Scattering, ETH Zurich and Paul Scherrer Institute, CH-5232 Villigen PSI, Switzerland
  • 6Department of Chemistry and Biochemistry, University of Bern, CH-3000 Bern 9, Switzerland
  • 7Institut Laue Langevin, BP 156, 38042 Grenoble Cedex 9, France

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Issue

Vol. 100, Iss. 20 — 23 May 2008

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