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Arresting of interfacial phase separation with an imposed flow

Ryuta X. Suzuki, Shoji Seya, Takahiko Ban, Manoranjan Mishra, and Yuichiro Nagatsu
Phys. Rev. Fluids 9, 024003 – Published 14 February 2024

Abstract

Using fluid displacement in a Hele-Shaw cell, we experimentally demonstrate the arresting effect of an imposed flow on a phase separation occurring in a growing liquid-liquid interfacial region, unlike in an initially homogeneous single-phase mixture quenched within the miscibility gap. Increasing the imposed flow rate reduces the exponent α in the form ΔAtα, where ΔA is the increase in the area occupied by the displacing fluid owing to phase separation. We show that α can be expressed as a function of the ratio of the phase separation rate to the flow rate on a single curve, indicating that the competition between the imposed flow and phase separation rates determines the degree of the interfacial phase separation. The arresting effect and the mechanism are verified by a numerical simulation.

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  • Received 16 August 2022
  • Accepted 5 January 2024

DOI:https://doi.org/10.1103/PhysRevFluids.9.024003

©2024 American Physical Society

Physics Subject Headings (PhySH)

Fluid DynamicsInterdisciplinary Physics

Authors & Affiliations

Ryuta X. Suzuki1,2,*, Shoji Seya1, Takahiko Ban3, Manoranjan Mishra4, and Yuichiro Nagatsu1

  • 1Department of Chemical Engineering, Tokyo University of Agriculture and Technology, Naka-cho 2-24-16, Koganei, Tokyo 184-8588, Japan
  • 2PRESTO, Japan Science and Technology Agency, Kawaguchi, Saitama 332-0012, Japan
  • 3Division of Chemical Engineering, Department of Materials Engineering Science, Graduate School of Engineering Science, Osaka University, Machikaneyamacho 1-3, Toyonaka City, Osaka 560-8531, Japan
  • 4Department of Mathematics, Indian Institute of Technology Ropar, Rupnagar 140001, India

  • *Corresponding author: ryuta.x.suzuki@gmail.com

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Vol. 9, Iss. 2 — February 2024

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