Abstract
Electron capture (EC) decay of a atom, the rate of which is affected by the electron density at the nucleus, forms a atom and emits a neutrino. Herein, we studied the EC decay rate of , in which those fullerenes have enhanced stability relative to their near neighbors, by using ab initio calculations. The stable and metastable atom sites and electron density at the nucleus in were calculated. Unlike , the nucleus sites in are always off center and close to the fullerene cage. Due to the bonding interaction between and the fullerene cage, the electron density at the nucleus in is smaller than those of a single atom and of in , leading to the result that the half-life of in increases. Based on equilibrium statistical thermodynamic calculations, the temperature effect on the half-life of has been analyzed. In contrast to , the temperature only slightly influences the half-life of in suggesting that the EC decay rate of could be precisely modified by using small fullerene cages.
- Received 19 June 2023
- Revised 30 August 2023
- Accepted 12 September 2023
DOI:https://doi.org/10.1103/PhysRevC.108.054604
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