Abstract
Adsorption of onto the Si(111)---Au surface with a high density of domain walls and its In-induced modification, a domain-wall-free Si(111)-(Au,In) surface, has been studied using scanning tunneling microscopy (STM). Adsorbed have been found to form close-packed hexagonal arrays displaying specific patterns of having different dim-bright STM contrast. On the Si(111)---Au surface, the dim-bright pattern replicates the domain-wall network of the substrate surface and has plausibly an electronic origin. On the homogeneous Si(111)-(Au,In) surface, a Moiré pattern of a two-dimensional lattice develops, which indicates periodic occupation of the same regular adsorption sites on the surface. Here, the dim-bright contrast is associated plausibly with different topographic heights of the molecules. In the case of the multilayer films, the dim-bright patterns of the first monolayer have been found to be inherited with gradual smearing in the next layers.
2 More- Received 26 January 2011
DOI:https://doi.org/10.1103/PhysRevB.83.195421
©2011 American Physical Society