Low-temperature thermal and optical properties of single-grained decagonal Al-Ni-Co quasicrystals

A. D. Bianchi, F. Bommeli, E. Felder, M. Kenzelmann, M. A. Chernikov, L. Degiorgi, H. R. Ott, and K. Edagawa
Phys. Rev. B 58, 3046 – Published 1 August 1998
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Abstract

We report measurements of the specific heat Cp(T) and of the thermal conductivities λp(T) along the periodic direction and λq(T) along a direction in the quasiperiodic plane for decagonal Al-Ni-Co at low temperatures. The coefficient γ=0.63 mJ mol1 K2 of the linear term to Cp(T) indicates a low density of electronic states at EF. The magnitude of the cubic-in-T term to the low-temperature specific heat is in fair agreement with the acoustic contribution to Cp(T) calculated from the results of low-temperature measurements of the elastic stiffness constants cij. The phonon contribution to λp(T) shows a distinct maximum at 25 K, typical for periodic crystals. The dominant feature in the phonon contribution to λq(T) is an extended plateau between 30 and 70 K, in agreement with the concept of generalized Umklapp processes in quasicrystals. This distinct difference between the phonon contributions to λp(T) and λq(T) is similar to that previously observed for Al65Cu20Co15. The optical conductivity σ1(ω) is obtained from reflectivity data in the frequency range between 1 meV and 12 eV. At low frequencies the optical conductivity σ1(ω) is characterized by an anisotropic Drude contribution. At high frequencies an additional absorption for the periodic and the quasiperiodic direction is observed centered at approximately 1 and 2 eV, respectively, which can be associated with electronic excitations across a pseudogap.

  • Received 25 November 1997

DOI:https://doi.org/10.1103/PhysRevB.58.3046

©1998 American Physical Society

Authors & Affiliations

A. D. Bianchi, F. Bommeli, E. Felder, M. Kenzelmann, M. A. Chernikov, L. Degiorgi, and H. R. Ott

  • Laboratorium für Festkörperphysik, Eidgenössische Technische Hochschule-Hönggerberg, CH-8093 Zürich, Switzerland

K. Edagawa

  • Institute of Industrial Science, University of Tokyo, Tokyo 106, Japan

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Issue

Vol. 58, Iss. 6 — 1 August 1998

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