Skyrmion alignment and pinning effects in the disordered multiphase skyrmion material Co8Zn8Mn4

M. E. Henderson, M. Bleuel, J. Beare, D. G. Cory, B. Heacock, M. G. Huber, G. M. Luke, M. Pula, D. Sarenac, S. Sharma, E. M. Smith, K. Zhernenkov, and D. A. Pushin
Phys. Rev. B 106, 094435 – Published 29 September 2022

Abstract

Underlying disorder in skyrmion materials may both inhibit and facilitate skyrmion reorientations and changes in topology. The identification of these disorder-induced topologically active regimes is critical to realizing robust skyrmion spintronic implementations, yet few studies exist for disordered bulk samples. Here, we employ small-angle neutron scattering (SANS) and micromagnetic simulations to examine the influence of skyrmion order on skyrmion lattice formation, transition, and reorientation dynamics across the phase space of a disordered polycrystalline Co8Zn8Mn4 bulk sample. Our measurements reveal a disordered-to-ordered skyrmion square lattice transition pathway characterized by the promotion of fourfold order in SANS and accompanied by a change in topology of the system, reinforced through micromagnetic simulations. Pinning responses are observed to dominate skyrmion dynamics in the metastable triangular lattice phase, enhancing skyrmion stabilization through a remarkable skyrmion memory effect which reproduces previous ordering processes and persists in zero field. These results uncover the cooperative interplay of anisotropy and disorder in skyrmion formation and restructuring dynamics, establishing tunable pathways for skyrmion manipulation.

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  • Received 27 April 2022
  • Revised 26 July 2022
  • Accepted 6 September 2022

DOI:https://doi.org/10.1103/PhysRevB.106.094435

©2022 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

M. E. Henderson1,2,*, M. Bleuel3,4, J. Beare5, D. G. Cory1,6, B. Heacock3, M. G. Huber3, G. M. Luke5,7, M. Pula5, D. Sarenac1, S. Sharma5, E. M. Smith5, K. Zhernenkov1,8, and D. A. Pushin1,2,†

  • 1Institute for Quantum Computing, University of Waterloo, Waterloo, Ontario, Canada N2L3G1
  • 2Department of Physics & Astronomy, University of Waterloo, Waterloo, Ontario, Canada N2L3G1
  • 3National Institute of Standards and Technology, Gaithersburg, Maryland 20899-8970, USA
  • 4Department of Materials Science and Engineering, University of Maryland, College Park, Maryland 20742-2115, USA
  • 5Department of Physics and Astronomy, McMaster University, Hamilton, Ontario, Canada L8S 4M1
  • 6Department of Chemistry, University of Waterloo, Waterloo, Ontario, Canada N2L3G1
  • 7Brockhouse Institute for Materials Research, Hamilton, Ontario, Canada L8S 4M1
  • 8Jülich Centre for Neutron Science at Heinz Maier-Leibnitz Zentrum, Forschungszentrum Jülich GmbH, 85748 Garching, Germany

  • *Corresponding author: mehenderson@uwaterloo.ca
  • Corresponding author: dmitry.pushin@uwaterloo.ca

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Issue

Vol. 106, Iss. 9 — 1 September 2022

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