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Orientation of molecules via laser-induced antialignment

E. Gershnabel, I. Sh. Averbukh, and Robert J. Gordon
Phys. Rev. A 73, 061401(R) – Published 8 June 2006

Abstract

We show that field-free molecular orientation induced by a half-cycle pulse may be considerably enhanced by an additional laser pulse inducing molecular antialignment. Two qualitatively different enhancement mechanisms are identified, depending on the pulse order, and their effects are optimized with the help of quasiclassical as well as fully quantum models.

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  • Received 12 September 2005

DOI:https://doi.org/10.1103/PhysRevA.73.061401

©2006 American Physical Society

Authors & Affiliations

E. Gershnabel and I. Sh. Averbukh

  • Department of Chemical Physics, Weizmann Institute of Science, Rehovot 76100, Israel

Robert J. Gordon

  • Department of Chemistry, University of Illinois at Chicago, Chicago, Illinois 60680, USA

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Issue

Vol. 73, Iss. 6 — June 2006

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