The optogalvanic effect induced in a Hg-Ar discharge by light at 546.1 nm is studied experimentally and theoretically. The plasma and its response to a disturbance in the atomic-level populations are described entirely in terms of electron collision cross sections and other fundamental parameters. In a detailed description of the laser interaction with the atomic system, it was necessary to take into account velocity-changing collisions (VCC). These collisions (VCC) strongly modify the interaction between the Doppler-broadened system and the optical field. In some Doppler-free optogalvanic spectra the dramatic influence of VCC on the velocity distribution of atomic-level population is evident. Measurements of the magnitude of the optogalvanic signal confirm most of the theoretical results. Some anomalous features of the impedance change due to a weak beam were observed when a strong counterpropagating beam was introduced.

• Received 15 May 1987

DOI:https://doi.org/10.1103/PhysRevA.36.5713