Abstract
A classical analysis of time correlations in simple fluids based on the generalized Langevin equation is presented. Formulas for the current-current correlations are developed explicitly in a region of frequencies ( ) and wave numbers ( ) which are explored in typical slow-neutron-scattering measurements. Where applicable, comparisons are made with the results of the numerical calculations of Rahman in argonlike liquids, and good agreement is generally found. The analysis is based on a hydrodynamic description of fluids involving frequency- and wavelength-dependent transport parameters. The frequency and wavelength dependence of shear and longitudinal viscosities are given explicitly for argon-like liquids.
- Received 21 November 1969
DOI:https://doi.org/10.1103/PhysRevA.2.962
©1970 American Physical Society