Universality of the Nonphononic Vibrational Spectrum across Different Classes of Computer Glasses

David Richard, Karina González-López, Geert Kapteijns, Robert Pater, Talya Vaknin, Eran Bouchbinder, and Edan Lerner
Phys. Rev. Lett. 125, 085502 – Published 19 August 2020
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Abstract

It has been recently established that the low-frequency spectrum of simple computer glass models is populated by soft, quasilocalized nonphononic vibrational modes whose frequencies ω follow a gapless, universal distribution D(ω)ω4. While this universal nonphononic spectrum has been shown to be robust to varying the glass history and spatial dimension, it has so far only been observed in simple computer glasses featuring radially symmetric, pairwise interaction potentials. Consequently, the relevance of the universality of nonphononic spectra seen in simple computer glasses to realistic laboratory glasses remains unclear. Here, we demonstrate the emergence of the universal ω4 nonphononic spectrum in a broad variety of realistic computer glass models, ranging from tetrahedral network glasses with three-body interactions, through molecular glasses and glassy polymers, to bulk metallic glasses. Taken together with previous observations, our results indicate that the low-frequency nonphononic vibrational spectrum of any glassy solid quenched from a melt features the universal ω4 law, independently of the nature of its microscopic interactions.

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  • Received 12 May 2020
  • Revised 9 July 2020
  • Accepted 21 July 2020

DOI:https://doi.org/10.1103/PhysRevLett.125.085502

© 2020 American Physical Society

Physics Subject Headings (PhySH)

Polymers & Soft MatterStatistical Physics & ThermodynamicsCondensed Matter, Materials & Applied Physics

Authors & Affiliations

David Richard1,*, Karina González-López1,*, Geert Kapteijns1, Robert Pater1, Talya Vaknin2, Eran Bouchbinder2, and Edan Lerner1

  • 1Institute for Theoretical Physics, University of Amsterdam, Science Park 904, 1098 XH Amsterdam, The Netherlands
  • 2Chemical and Biological Physics Department, Weizmann Institute of Science, Rehovot 7610001, Israel

  • *These authors contributed equally to this work.

See Also

Universal Low-Frequency Vibrational Modes in Silica Glasses

Silvia Bonfanti, Roberto Guerra, Chandana Mondal, Itamar Procaccia, and Stefano Zapperi
Phys. Rev. Lett. 125, 085501 (2020)

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Vol. 125, Iss. 8 — 21 August 2020

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