Local Weak Ferromagnetism in Single-Crystalline Ferroelectric BiFeO3

M. Ramazanoglu, M. Laver, W. Ratcliff, II, S. M. Watson, W. C. Chen, A. Jackson, K. Kothapalli, Seongsu Lee, S.-W. Cheong, and V. Kiryukhin
Phys. Rev. Lett. 107, 207206 – Published 11 November 2011

Abstract

Polarized small-angle neutron scattering studies of single-crystalline multiferroic BiFeO3 reveal a long-wavelength spin density wave generated by 1° spin canting of the spins out of the rotation plane of the antiferromagnetic cycloidal order. This signifies weak ferromagnetism within mesoscopic regions of dimension 0.03 microns along [11¯0], to several microns along [111], confirming a long-standing theoretical prediction. The average local magnetization is 0.06μB/Fe. Our results provide an indication of the intrinsic macroscopic magnetization to be expected in ferroelectric BiFeO3 thin films under strain, where the magnetic cycloid is suppressed.

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  • Received 26 July 2011

DOI:https://doi.org/10.1103/PhysRevLett.107.207206

© 2011 American Physical Society

Authors & Affiliations

M. Ramazanoglu1, M. Laver2,3,4, W. Ratcliff, II5, S. M. Watson5, W. C. Chen4,5, A. Jackson4,5, K. Kothapalli4,5, Seongsu Lee6, S.-W. Cheong1, and V. Kiryukhin1

  • 1Department of Physics and Astronomy, Rutgers University, Piscataway, New Jersey 08854, USA
  • 2Materials Research Division, Risø DTU, Technical University of Denmark, DK-4000 Roskilde, Denmark
  • 3Nano Science Center, Niels Bohr Institute, University of Copenhagen, DK-2100 Copenhagen, Denmark
  • 4Department of Materials Science and Engineering, University of Maryland, College Park, Maryland 20742, USA
  • 5NIST Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899, USA
  • 6Neutron Science Division, Korea Atomic Research Institute, Daejon 305-353, Korea

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Issue

Vol. 107, Iss. 20 — 11 November 2011

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