Abstract
We have deduced the emission probability of the 447-keV ray from the decay of (9.0 h) relative to that of the 254-keV ray from the (34.4 h) decay in transient equilibrium. The time-dependent factor in transient equilibrium was applied following the Bateman equation for a radioactive decay chain. The isotope was produced via the reaction by bombarding with a proton beam from the 88-in. cyclotron at Lawrence Berkeley National Laboratory. -ray intensities were measured using an HPGe detector. The emission probability for the 447-keV ray deduced in this work is 1.21(3) (that is 1.21 ± 0.03) per hundred parent decays, which differs significantly from an earlier published value of 2.24(10). We identify the source of this discrepancy to be an incorrect use of the time-dependent factor. Additionally, we have deduced the emission probability of the 504-keV ray from the decay of (2.68 h) relative to that of the 232-keV ray from the (1.127 h) decay in transient equilibrium. The isotope was produced via the reaction by bombarding with a proton beam at the same facility. The study confirms the assumption of the time-dependent correction for recommending the emission probability of the 504-keV ray in the literature. Our work highlights the importance of explicit description by authors of any time-dependent correction they have made when reporting -ray intensities for nuclides in transient equilibrium. The need and significance of accurate and precise decay data of and in basic science and medicine is briefly outlined.
- Received 13 September 2019
- Revised 28 January 2020
- Accepted 11 May 2020
DOI:https://doi.org/10.1103/PhysRevC.101.064619
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