Anisotropic superconductivity and magnetism in single-crystal RbEuFe4As4

M. P. Smylie, K. Willa, J.-K. Bao, K. Ryan, Z. Islam, H. Claus, Y. Simsek, Z. Diao, A. Rydh, A. E. Koshelev, W.-K. Kwok, D. Y. Chung, M. G. Kanatzidis, and U. Welp
Phys. Rev. B 98, 104503 – Published 5 September 2018

Abstract

We investigate the anisotropic superconducting and magnetic properties of single-crystal RbEuFe4As4 using magnetotransport and magnetization measurements. We determine a magnetic ordering temperature of the Eu moments of Tm=15K and a superconducting transition temperature of Tc=36.8K. The superconducting phase diagram is characterized by high upper critical field slopes of 70 and 42 kG/K for in-plane and out-of-plane fields, respectively, and a surprisingly low superconducting anisotropy of Γ=1.7. Ginzburg-Landau parameters of κc67 and κab108 indicate extreme type-II behavior. These superconducting properties are in line with those commonly seen in optimally doped Fe-based superconductors. In contrast, Eu magnetism is quasi-two dimensional (2D), as evidenced by highly anisotropic in-plane and out-of-plane exchange constants of 0.6 K and <0.04 K. A consequence of the quasi-2D nature of the Eu magnetism are strong magnetic fluctuation effects, a large suppression of the magnetic ordering temperature as compared to the Curie-Weiss temperature, and a kinklike anomaly in the specific heat devoid of any singularity. Magnetization curves reveal a clear magnetic easy-plane anisotropy with in-plane and out-of-plane saturation fields of 2 and 4 kG.

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  • Received 11 May 2018

DOI:https://doi.org/10.1103/PhysRevB.98.104503

©2018 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

M. P. Smylie1,2, K. Willa1, J.-K. Bao1, K. Ryan3, Z. Islam4, H. Claus1, Y. Simsek1, Z. Diao5,6, A. Rydh6, A. E. Koshelev1, W.-K. Kwok1, D. Y. Chung1, M. G. Kanatzidis1,7, and U. Welp1

  • 1Materials Science Division, Argonne National Laboratory, 9700 S. Cass Avenue, Argonne, Illinois 60439, USA
  • 2Department of Physics, University of Notre Dame, Notre Dame, Indiana 46556, USA
  • 3Department of Physics, University of Illinois at Urbana-Champaign, Urbana, Illinois 61801, USA
  • 4Advanced Photon Source, Argonne National Laboratory, 9700 S. Cass Avenue, Lemont, Illinois 60439, USA
  • 5Laboratory of Mathematics, Physics and Electrical Engineering, Halmstad University, SE-301 18 Halmstad, Sweden
  • 6Department of Physics, Stockholm University, SE-106 91 Stockholm, Sweden
  • 7Department of Chemistry, Northwestern University, Evanston, Illinois 60208, USA

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Issue

Vol. 98, Iss. 10 — 1 September 2018

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