Effects of the individual particle relaxation time on superspin glass dynamics

Mikael Svante Andersson, Jose Angel De Toro, Su Seong Lee, Peter S. Normile, Per Nordblad, and Roland Mathieu
Phys. Rev. B 93, 054407 – Published 8 February 2016

Abstract

The low temperature dynamic magnetic properties of two dense magnetic nanoparticle assemblies with similar superspin glass transition temperatures Tg140 K are compared. The two samples are made from batches of 6 and 8 nm monodisperse γFe2O3 nanoparticles, respectively. The properties of the individual particles are extracted from measurements on reference samples where the particles have been covered with a thick silica coating. The blocking temperatures of these dilute assemblies are found at 12.5 K for the 6 nm particles and at 35 K for the 8 nm particles, which implies different anisotropy energy barriers of the individual particles and vastly different temperature evolution of their relaxation times. The results of the measurements on the concentrated particle assemblies suggest a strong influence of the particle energy barrier on the details of the aging dynamics, memory behavior, and apparent superspin dimensionality of the particles.

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  • Received 21 December 2015

DOI:https://doi.org/10.1103/PhysRevB.93.054407

©2016 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Mikael Svante Andersson1,*, Jose Angel De Toro2, Su Seong Lee3, Peter S. Normile2, Per Nordblad1, and Roland Mathieu1

  • 1Department of Engineering Sciences, Uppsala University, Box 534, SE-751 21 Uppsala, Sweden
  • 2Instituto Regional de Investigación Científica Aplicada (IRICA) and Departamento de Física Aplicada, Universidad de Castilla-La Mancha 13071 Ciudad Real, Spain
  • 3Institute of Bioengineering and Nanotechnology, 31 Biopolis Way, The Nanos, Singapore 138669, Singapore

  • *Mikael.Andersson@angstrom.uu.se

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Vol. 93, Iss. 5 — 1 February 2016

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