Correlation of optical conductivity and angle-resolved photoemission spectra of strong-coupling large polarons and its display in cuprates

A. E. Myasnikova and E. N. Myasnikov
Phys. Rev. B 77, 165136 – Published 30 April 2008

Abstract

A common approach is used to calculate a band due to strong-coupling large polaron (SCLP) photodissociation in angle-resolved photoemission spectroscopy (ARPES) and in optical conductivity (OC) spectra. It is based on using the coherent-state representation for the phonon field in SCLP. The calculated positions of both band maxima are universal functions of one parameter—the SCLP binding energy Ep: a maximum of the band in the ARPES spectrum lies at a carrier binding energy of about 3.2Ep; the OC band maximum is at a photon energy of about 4.2Ep. The half-widths of the bands are mainly determined by Ep and slightly depend on the electron-phonon coupling constant α; for α=68, the half-width of the band in the ARPES spectrum is 1.71.3Ep and the OC band half-width is 2.82.2Ep. By using these results, one can predict the approximate maximum position and half-width of the band in the ARPES spectrum from the maximum of the mid-IR OC band and vice versa. Comparison of the results with experiments leads to the conclusion that underdoped cuprates contain SCLPs with Ep=0.10.2eV, which is in good conformity with the medium parameters in cuprates. The values of the polaron binding energy determined from experimental ARPES and OC spectra of the same material are in good conformity, too: the difference between them is within 10%.

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  • Received 15 December 2007

DOI:https://doi.org/10.1103/PhysRevB.77.165136

©2008 American Physical Society

Authors & Affiliations

A. E. Myasnikova and E. N. Myasnikov

  • South Federal University, 344090 Rostov-on-Don, Russia

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Issue

Vol. 77, Iss. 16 — 15 April 2008

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