X-ray magnetic circular dichroism study of uranium/iron multilayers

F. Wilhelm, N. Jaouen, A. Rogalev, W. G. Stirling, R. Springell, S. W. Zochowski, A. M. Beesley, S. D. Brown, M. F. Thomas, G. H. Lander, S. Langridge, R. C. C. Ward, and M. R. Wells
Phys. Rev. B 76, 024425 – Published 18 July 2007

Abstract

X-ray magnetic circular dichroism (XMCD) measurements were performed at the U M4,5 edges and Fe K edge on well-defined uranium/iron multilayers with different compositions. The multilayers have layer thicknesses in the range 940Å for uranium and 934Å for iron. At both 10K and room temperature, the U layers are magnetically polarized in all of the multilayers studied. To deduce the magnetic moment on the uranium from the XMCD results requires assumptions about the magnetic dipole operator TZ in the analysis, and this is discussed in detail. Given the most likely scenario of strong hybridization between the U5f and Fe3d states, the largest value of the induced U moment is 0.12μB, which is located primarily at the interface and oscillates within the uranium layer.

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  • Received 30 March 2006

DOI:https://doi.org/10.1103/PhysRevB.76.024425

©2007 American Physical Society

Authors & Affiliations

F. Wilhelm, N. Jaouen, A. Rogalev, and W. G. Stirling*

  • European Synchrotron Radiation Facility, Boîte Postale 220, F-38043 Grenoble Cedex, France

R. Springell and S. W. Zochowski

  • Department of Physics and Astronomy, University College London, London WC1E 6BT, United Kingdom

A. M. Beesley, S. D. Brown, and M. F. Thomas

  • Department of Physics, University of Liverpool, Liverpool L69 7ZE, United Kingdom

G. H. Lander

  • Institute for Transuranium Elements, European Commission, JRC, Postfach 2340, 76125 Karlsruhe, Germany

S. Langridge

  • Rutherford Appleton Laboratory, Chilton, Didcot, Oxon OX11 0QX, United Kingdom

R. C. C. Ward and M. R. Wells

  • Clarendon Laboratory, University of Oxford, Oxford, Oxon OX1 3PU, United Kingdom

  • *Also at Department of Physics, University of Liverpool, Liverpool L69 7ZE, United Kingdom.

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Issue

Vol. 76, Iss. 2 — 1 July 2007

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