Measuring the phonon-assisted spectral function by using a nonequilibrium three-terminal single-molecular device

Juntao Song, Qing-feng Sun, Jinhua Gao, and X. C. Xie
Phys. Rev. B 75, 195320 – Published 17 May 2007

Abstract

The electron transport through a three-terminal single-molecular transistor (SMT) is theoretically studied. We find that the differential conductance of the third and weakly coupled terminal versus its voltage matches well with the spectral function versus the energy when certain conditions are met. Particularly, this excellent matching is maintained even for the complicated structure of the phonon-assisted side peaks. Thus, this device offers an experimental approach to explore the shape of the phonon-assisted spectral function in detail. In addition, we discuss the conditions of a perfect matching. The results show that at low temperatures, the matching survives regardless of the bias and the energy levels of the SMT. However, at high temperatures, the matching is destroyed.

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  • Received 29 December 2006

DOI:https://doi.org/10.1103/PhysRevB.75.195320

©2007 American Physical Society

Authors & Affiliations

Juntao Song1, Qing-feng Sun1,*, Jinhua Gao1, and X. C. Xie1,2

  • 1Beijing National Laboratory for Condensed Matter Physics and Institute of Physics, Chinese Academy of Sciences, Beijing 100080, China
  • 2Department of Physics, Oklahoma State University, Stillwater, Oklahoma 74078, USA

  • *Electronic address: sunqf@aphy.iphy.ac.cn

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Issue

Vol. 75, Iss. 19 — 15 May 2007

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