The magnetic anisotropy energy (MAE) of face-centered-tetragonal (fct) Ni is calculated as a function of the axial c/a ratio. It is shown that the MAE for fct Ni is tremendously enhanced relative to the MAE for fcc Ni. The theoretical results are compared with measurements done by means of ferromagnetic resonance on fct Ni films grown on a Cu(001) substrate. Both experiment and theory show that the tetragonal distortion of Ni is crucial for the understanding of the transition to the out-of-plane magnetization for Ni films on Cu(001) for thicknesses above ∼ 7 atomic monolayers. We have also calculated the magnetostrictive constants for fcc Ni and obtained ${\lambda }_{001}$=-245×${10}^{\mathrm{-}6}$ and ${\lambda }_{111}$=-110×${10}^{\mathrm{-}6}$. The relation between ${\lambda }_{001}$ and the MAE of fct Ni is investigated by means of magnetoelastic theory as well as by first principles calculations.

• Received 28 October 1996

DOI:https://doi.org/10.1103/PhysRevB.55.15026