Abstract
Dynamics of large- acoustic phonons and low-frequency optical phonons in La are investigated. Monoenergetic nonequilibrium phonons are obtained by electron-phonon relaxation of laser-excited ions and are detected with phonon-induced absorption of the anti-Stokes vibronic sideband of the state of . Monoenergetic phonon occupation numbers of are observed and the decay of these nonequilibrium phonons is interpreted with the aid of estimates of some of the parameters of the electron-phonon system. We conclude that the observed decay is dominated by anharmonic breakup of low-frequency optical phonons, which have recently been seen with inelastic neutron scattering in the (41-54)- phonon-energy range of these experiments. Lifetimes in the 10-ns range are obtained, consistent with some theoretical estimates.
- Received 25 April 1983
DOI:https://doi.org/10.1103/PhysRevB.28.4786
©1983 American Physical Society