Manipulation of two-photon-induced fluorescence spectra of chromophore aggregates with entangled photons: A simulation study

Frank Schlawin, Konstantin E. Dorfman, Benjamin P. Fingerhut, and Shaul Mukamel
Phys. Rev. A 86, 023851 – Published 29 August 2012

Abstract

The nonclassical spectral and temporal features of entangled photons offer new possibilities to investigate the interactions of excitons in photosynthetic complexes and to target the excitation of specific states. Simulations of fluorescence in the bacterial reaction center induced by entangled light demonstrate a degree of selectivity of double-exciton states which is not possible using classical stochastic light with the same power spectrum.

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  • Received 19 April 2012

DOI:https://doi.org/10.1103/PhysRevA.86.023851

©2012 American Physical Society

Authors & Affiliations

Frank Schlawin, Konstantin E. Dorfman, Benjamin P. Fingerhut, and Shaul Mukamel*

  • Department of Chemistry, University of California, Irvine, California 92697-2025, USA

  • *smukamel@uci.edu

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Issue

Vol. 86, Iss. 2 — August 2012

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