Abstract
In this paper the phase-dependent features of ultrashort laser pulse resonant propagation in a two-level dipolar molecule are demonstrated by solving full Maxwell–Bloch equations. The electronic properties of dipolar molecule 4-trans-[p-(N, N-Di-n-butylamino)-p -stilbenylvinyl] pyridine (DBASVP) molecule, one-dimensional asymmetric organic molecule, is calculated by density functional theory at ab initio level. The numerical results show that the carrier propagation and the spectrum evolution of the pulse are sensitive to its initial phase and the phase sensitivity is more obvious for larger area pulse. The phase-dependent feature is more evident in dipolar molecule because the permanent dipole moment makes the nonlinear effects stronger.