Resonant nonlinear optical properties of PbS nanocrystals under nano- and picosecond pulsed laser excitation

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, , Citation Jochen Fick et al 1997 Pure Appl. Opt. 6 527 DOI 10.1088/0963-9659/6/5/004

0963-9659/6/5/527

Abstract

Using the sol-gel technique we have investigated PbS-doped thin films. The resonant nonlinear refractive index of these samples was measured, using two different techniques: nonlinear m-lines and degenerate four-wave mixing (DFWM). The measured values of the nonlinear refractive index are and for the m-lines and DFWM, respectively. We explain this difference as being due to the different durations of the laser pulses used (7 ns for m-lines and 30 ps for DFWM).

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10.1088/0963-9659/6/5/004